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学者姓名：杨文斌
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Abstract ：
This study develops a functionalization strategy for incorporating cellulose nanocrystals (CNCs) into unsaturated polyester resin (UPR) to simultaneously enhance its strength and toughness. Surface modification of CNCs was achieved through sequential reactions with toluene diisocyanate (TDI) and hydroxyethyl acrylate (HEA), introducing carbon double bonds(C=C) to obtain modified CNC (m-CNC). The m-CNC was subsequently compounded with UPR to fabricate composite materials. A comprehensive investigation of the composites' morphological features, mechanical performance, and thermal behavior was conducted through transmission electron microscopy (TEM), mechanical testing, dynamic mechanical analysis (DMA), and thermogravimetric analysis (TGA). Experimental results demonstrate that 0.3 wt% m-CNC incorporation markedly improves UPR's mechanical properties, with the composite exhibiting 23.55% higher tensile strength, 59.01% increased flexural strength, and 96.16% enhanced impact resistance compared to unmodified UPR. DMA characterization revealed that covalent cross-linking between m-CNC and the UPR matrix restricts polymer chain mobility, resulting in a 35.4% elevation in storage modulus. TGA data confirmed the heat resistance improvement, showing 12.8 degrees C and 9.3 degrees C increases in thermal decomposition temperatures for m-CNC/UPR composites relative to pure UPR and unmodified CNCs/UPR systems, respectively. This synergistic modification approach effectively balances structural integrity preservation of CNCs with significant enhancement of UPR's multifunctional performance, demonstrating potential applications in automotive, construction, new energy, and eco-friendly packaging industries. It emerges as a promising alternative to conventional composite materials.
Keyword ：
cellulose nanocrystal modification cellulose nanocrystal modification interfacial covalent cross-linking interfacial covalent cross-linking nanocomposites nanocomposites synergistic mechanical enhancement synergistic mechanical enhancement unsaturated polyester resin unsaturated polyester resin
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| GB/T 7714 | Li, Ran , Feng, Lifei , Yang, Wenbin et al. Sequential Isocyanate/Acrylate Functionalization of Cellulose Nanocrystals for Multi-Performance Advancement in Unsaturated Polyester Composites [J]. | POLYMER COMPOSITES , 2025 . |
| MLA | Li, Ran et al. "Sequential Isocyanate/Acrylate Functionalization of Cellulose Nanocrystals for Multi-Performance Advancement in Unsaturated Polyester Composites" . | POLYMER COMPOSITES (2025) . |
| APA | Li, Ran , Feng, Lifei , Yang, Wenbin , Lin, Huiping , Wu, Yiqiang . Sequential Isocyanate/Acrylate Functionalization of Cellulose Nanocrystals for Multi-Performance Advancement in Unsaturated Polyester Composites . | POLYMER COMPOSITES , 2025 . |
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Glass fiber-reinforced polymer (GFRP) composites were prepared by hand lay-up using unsaturated polyester resin (UPR) matrices in which a hyperbranched polyester (HBP) synthesized via a polyethylene glycol (PEG) core route was incorporated. Glass fibers (GFs) were functionalized to create "rigid" (HEA/TDI-modified, m-GF) and "flexible" (KH570-modified, KH570-GF) interfaces. HBP-modified UPR composites exhibited enhanced tensile, flexural, and impact strengths by 62.2%, 17.5%, and 95.0%, respectively, versus unmodified counterparts. Introducing the rigid m-GF interface further amplified these improvements, achieving strength gains of 96.1% (tensile), 90.9% (flexural), and 80.4% (impact). The flexible KH570-GF interface yielded the most pronounced synergistic effect: the optimum system (KH570-GF + 5 wt% HBP) achieved a tensile strength of 336.8 MPa (a 113% increase), a flexural strength of 622.1 MPa (93.6% increase), and an impact strength of 142.2 kJ m-2 (187% increase) relative to the baseline GF/UPR composite. Dynamic mechanical analysis confirmed increased glass transition temperatures, indicating enhanced thermal stability from improved crosslinking. Scanning electron microscopy demonstrated reduced fiber-matrix debonding and suppressed crack propagation in the modified systems. The rigid interface primarily enhanced load transfer efficiency, whereas the flexible interface promoted energy absorption via interfacial slippage. These findings illustrate that independent tailoring of rigid or flexible interfaces provides distinct pathways for performance optimization, effectively overcoming the traditional strength-toughness trade-off in GFRPs and offering customizable solutions for aerospace and structural applications.
Keyword ：
glass fiber-reinforced composites glass fiber-reinforced composites hyperbranched polyester hyperbranched polyester interface modification interface modification interfacial engineering interfacial engineering mechanical properties mechanical properties
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| GB/T 7714 | Li, Ran , Chen, Shanwei , Yang, Wenbin et al. Dual Interfacial Engineering of Glass Fiber-Reinforced Composites: Synergistic Enhancement via Hyperbranched Polyester-Modified Resin and Rigid/Flexible Fiber Coatings [J]. | POLYMER COMPOSITES , 2025 . |
| MLA | Li, Ran et al. "Dual Interfacial Engineering of Glass Fiber-Reinforced Composites: Synergistic Enhancement via Hyperbranched Polyester-Modified Resin and Rigid/Flexible Fiber Coatings" . | POLYMER COMPOSITES (2025) . |
| APA | Li, Ran , Chen, Shanwei , Yang, Wenbin , Lin, Huiping , Wu, Yiqiang . Dual Interfacial Engineering of Glass Fiber-Reinforced Composites: Synergistic Enhancement via Hyperbranched Polyester-Modified Resin and Rigid/Flexible Fiber Coatings . | POLYMER COMPOSITES , 2025 . |
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重组竹材料内部存在微裂纹和层间空隙，高温处理后如果承受冲击荷载，容易发生断裂破坏，影响结构性能。选取3个无量纲裂缝长度(0.4,0.5,0.6)、5个含水率(4%,8%,10%,12%,16%)和6个试验温度(20,80,130,180,230,280℃)为参数，进行重组竹横纹直槽半圆盘试件三点弯曲断裂试验。为了对比加载率对重组竹横纹Ⅰ型断裂韧度的影响，通过分离式霍普金森压杆(SHPB)控制气压达到3种不同的加载速度，分别以冲击速度6,7,8 m/s为参数，分析断裂韧度随温度、含水率及冲击速度的变化规律，并提出了动力影响系数公式。试验结果表明：重组竹横纹Ⅰ型动态断裂韧度在相同无量纲裂纹长度和冲击速度下的变化趋势和准静态加载条件下基本相同，随着含水率由4%上升至16%,断裂韧度呈先上升后下降的趋势，在含水率为10%时断裂韧度最大；随着温度由20℃上升至280℃,断裂韧度呈逐渐下降趋势，当温度超过180℃时，部分试件的断裂韧度下降程度更为明显。通过研究重组竹在高温处理后的断裂力学特性，为重组竹材料的相关规范制定提供了理论基础，从而促进其在工程结构领域的广泛应用。
Keyword ：
Ⅰ型 Ⅰ型 断裂韧度 断裂韧度 重组竹 重组竹 霍普金森压杆(SHPB) 霍普金森压杆(SHPB) 高温处理 高温处理
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| GB/T 7714 | 吴前煌 , 郭任坤 , 郭楠 et al. 重组竹高温处理后的Ⅰ型断裂力学特性 [J]. | 林业工程学报 , 2025 , 10 (04) : 19-27 . |
| MLA | 吴前煌 et al. "重组竹高温处理后的Ⅰ型断裂力学特性" . | 林业工程学报 10 . 04 (2025) : 19-27 . |
| APA | 吴前煌 , 郭任坤 , 郭楠 , 饶久平 , 杨文斌 , 盛叶 . 重组竹高温处理后的Ⅰ型断裂力学特性 . | 林业工程学报 , 2025 , 10 (04) , 19-27 . |
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本发明公开了一种竹木加工处理方法及处理系统，本方案通过将竹纤维束置于振动床设备中进行翻动处理，同时，令其所在环境的真空度为101125～101225Pa，且使竹纤维束暴露在等离子体中，使得经处理后的竹纤维束在浸胶时，能够具有更优的复合能力；基于此，本方案提出了一种处理系统，其通过在真空等离子腔体内部设置振动床，在处理过程中使竹木质单元均匀翻滚，从而实现均匀的等离子体表面处理，提高处理效率，增强竹木质单元与树脂复合时的界面结合性能。
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| GB/T 7714 | 杨文斌 , 洪国隆 , 李燃 et al. 一种竹木加工处理方法及处理系统 : CN202411860771.8[P]. | 2024-12-17 . |
| MLA | 杨文斌 et al. "一种竹木加工处理方法及处理系统" : CN202411860771.8. | 2024-12-17 . |
| APA | 杨文斌 , 洪国隆 , 李燃 , 张欣向 , 陈寒娴 , 温柔 et al. 一种竹木加工处理方法及处理系统 : CN202411860771.8. | 2024-12-17 . |
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以杉木(Cunninghamia lanceolata)木材为研究对象，将木材裁切为20 mm×20 mm×12 mm(径向×弦向×纵向)的样品；以有机聚硅氮烷(OPSZ)、正己烷为试剂，按照质量比m(有机聚硅氮烷)∶m(正己烷)分别为1∶3、1∶5、1∶7、1∶9、1∶11的比例配制改性液；采用浸渍法将木材样品分别浸入不同比例的改性液中，常温(25℃)常压放置2 h后，将样品转移至烘箱中120℃热处理5 h,木材表面有机聚硅氮烷涂层固化，制得有机聚硅氮烷改性木材样品；应用相关仪器、参照国家相关标准及试验设计的方法，测定改性前后木材表面形貌与结构、木材表面化学成分与官能团变化、木材疏水性能与防水性能、涂层硬度、涂层机械稳定性、木材抗污性能、木材热稳定性，分析有机聚硅氮烷涂层的性能及其对木材保护的作用。结果表明：(1)采用扫描电镜观察改性前后木材的表面形貌，与未改性木材相比，经过有机聚硅氮烷改性的木材表面覆盖了一层较为致密的涂层。(2)采用傅里叶变换红外光谱仪、X射线光电子能谱仪对改性前后木材表面官能团和木材表面元素的变化分析表明，改性后木材表面引入了稳定性好的有机硅骨架以及疏水的甲基；有机聚硅氮烷显著提高了木材的疏水性和防水性能，木材的水接触角从72.0°增大至119.3°,24 h吸水率从79.00%显著下降至25.38%。(3)改性后木材对牛奶、咖啡、橙汁、可乐等常见污染物，具有良好的抗污性。(4)改性后，木材表面有机聚硅氮烷涂层的铅笔硬度达到6 H,并且能够经受长时间的机械摩擦，表明其具有优异的机械稳定性。(5)热质量分析表明，有机聚硅氮烷显著提升了木材的热稳定性。(6)综合试验结果，有机聚硅氮烷涂层具有良好的防水性、耐机械摩擦、热稳定性，可在严苛环境时的木材保护中应用。
Keyword ：
有机聚硅氮烷 有机聚硅氮烷 木材改性 木材改性 木材表面 木材表面 杉木 杉木 疏水涂层 疏水涂层
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| GB/T 7714 | 陈寒娴 , 张林昕 , 檀佳欣 et al. 杉木木材表面原位构筑坚固的疏水聚硅氮烷涂层 [J]. | 东北林业大学学报 , 2025 , 53 (04) : 140-147 . |
| MLA | 陈寒娴 et al. "杉木木材表面原位构筑坚固的疏水聚硅氮烷涂层" . | 东北林业大学学报 53 . 04 (2025) : 140-147 . |
| APA | 陈寒娴 , 张林昕 , 檀佳欣 , 王诗彤 , 温涛 , 林舒敏 et al. 杉木木材表面原位构筑坚固的疏水聚硅氮烷涂层 . | 东北林业大学学报 , 2025 , 53 (04) , 140-147 . |
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Phase change materials have excellent heat storage capacity, which is a great advantage in utilizing clean energy and improving the efficiency of energy use. However, the leakage issue of solid-liquid phase change materials limits their application. In this study, Arundo donax cv. Lvzhou No.1 (LZ1) was utilized to fabricate a porous biomass carbon skeleton, into which polyethylene glycol (PEG) was introduced via vacuum impregnation to address the PEG leakage issue during phase change and enhance thermal conductivity. The prepared shape-stabilized composite phase change material (ss-CPCM) was characterized and tested for its adsorption rate and thermal conductivity. The results of BET, SEM and leakage experiments showed that PEG can be well adsorbed in the pores of carbonized LZ1 (CLZ1). FT-IR and XRD analyses confirmed the physical interaction between PEG and CLZ1. The results of DSC and thermal conductivity tests yielded that the composite phase change material has a high latent heat value (134.74 J g(-1)), and its thermal conductivity was improved by about 78.12% compared with that of PEG. Thermogravimetric and thermal cycling experiments demonstrated that the prepared composite phase change materials have good thermal stability and still have good energy storage capacity after many thermal cycles. The prepared PEG/CLZ1 ss-CPCM is an economical, energy-saving and sustainable phase change material with potential applications in the field of building energy efficiency.
Keyword ：
Lvzhou No.1 biochar Lvzhou No.1 biochar Phase change materials Phase change materials Shape-stabilized Shape-stabilized Thermal conductivity Thermal conductivity Thermal performance analysis Thermal performance analysis
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| GB/T 7714 | Zhu, Kunyi , Xu, Qingliang , Xie, Jingzhou et al. Preparation of Lvzhou No.1 biomass carbon-based shape-stabilized composite phase change material and their thermal properties [J]. | JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY , 2025 , 150 (8) : 5991-6000 . |
| MLA | Zhu, Kunyi et al. "Preparation of Lvzhou No.1 biomass carbon-based shape-stabilized composite phase change material and their thermal properties" . | JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY 150 . 8 (2025) : 5991-6000 . |
| APA | Zhu, Kunyi , Xu, Qingliang , Xie, Jingzhou , Zhang, Xu , Rao, Jiuping , Yang, Wenbin et al. Preparation of Lvzhou No.1 biomass carbon-based shape-stabilized composite phase change material and their thermal properties . | JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY , 2025 , 150 (8) , 5991-6000 . |
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With the continuous growth of global building energy consumption, the development of efficient energy-storage building materials is of great significance to promote the sustainable development of the construction industry. In this study, Arundo donax cv. Lvzhou No.1 (LZ1) was chemically activated using KOH and H3PO4 to prepare two activated carbons, denoted as KALZ1 and PALZ1, respectively. These activated carbons were then used as supporting materials and loaded with capric acid-stearic acid eutectic mixture (CA-SA) using vacuum impregnation method. The resulting shape-stabilized phase change materials (SSPCMs) were designated as CA-SA/ KALZ1 and CA-SA/PALZ1, corresponding to their respective activated carbon carriers. PALZ1 exhibited superior encapsulation capability with a loading rate of 78.62 %, which was attributed to its larger specific surface area (318.46 m2/g) and uniform pore size (0.827 nm). The thermal conductivity of CA-SA/PALZ1 was 0.406 W/ (m & sdot;K), which was 98 % higher than the 0.205 W/(m & sdot;K) of pure CA-SA. Its latent heat value was 112.87 J/g, and only decreased by 6.50 J/g after 500 thermal cycles, showing excellent thermal performance and thermal stability. Furthermore, CA-SA/PALZ1 was added into phosphogypsum (PG) to prepare energy-storing PG-based composite. At a dosage of 15 wt%, the compressive strength and flexural strength of the composite were increased by 6.18 % and 12.12 % compared with the control group, respectively, with a latent heat value of 18.81 J/g. This study demonstrated the feasibility of using LZ1-based activated carbon as a phase-change material carrier. This strategy achieved synergistic value-addition of biomass resources and industrial by-products, providing insights for developing novel energy-efficient building materials.
Keyword ：
Activated carbon Activated carbon Arundo donax cv. Lvzhou No.1 Arundo donax cv. Lvzhou No.1 Phase change material Phase change material Phosphogypsum Phosphogypsum Thermal storage Thermal storage
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| GB/T 7714 | Xu, Qing , Zhu, Kunyi , Zhang, Xu et al. Comparative study of KOH and H3PO4 activated Lvzhou No. 1-based shape-stabilized phase change materials: Properties and potential application in phosphogypsum [J]. | CONSTRUCTION AND BUILDING MATERIALS , 2025 , 476 . |
| MLA | Xu, Qing et al. "Comparative study of KOH and H3PO4 activated Lvzhou No. 1-based shape-stabilized phase change materials: Properties and potential application in phosphogypsum" . | CONSTRUCTION AND BUILDING MATERIALS 476 (2025) . |
| APA | Xu, Qing , Zhu, Kunyi , Zhang, Xu , Yang, Wenbin , Rao, Jiuping , Liu, Mengmei . Comparative study of KOH and H3PO4 activated Lvzhou No. 1-based shape-stabilized phase change materials: Properties and potential application in phosphogypsum . | CONSTRUCTION AND BUILDING MATERIALS , 2025 , 476 . |
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天然植物纤维是一种绿色可再生资源，具有来源丰富、价格低廉、可生物降解、物化性能丰富可调等特点，已成为化学、材料等领域研究的热点。然而，由于天然植物纤维具有易吸湿、易受霉菌微生物侵害、与非极性聚合物界面相容性差等缺点，限制了天然植物纤维材料的高效和高附加值应用，有必要对其进行改性处理。原子转移自由基聚合(ATRP)是一种有别于传统意义上的自由基聚合法，因其活性可控、分子设计能力强，被广泛用于天然植物纤维材料功能化改性。本文结合作者课题组及国内外的研究情况，介绍了天然植物纤维ATRP改性的反应机理，归纳总结了近年来ATRP在竹木纤维、棉纤维、麻纤维以及其他植物纤维改性方面的研究进展，阐述了电子转移活化再生催化剂原子转移自由基聚合(ARGET ATRP)在植物纤维功能化改性中优势及发展应用，其能够提高接枝聚合物复合材料的疏水性、疏水耐久性，提高复合材料的生物相容性、抗菌性和吸附性等生物性能，并且还能提升复合材料的力学性能。最后对天然植物纤维ATRP改性面临的问题进行了总结并展望了其发展前景。
Keyword ：
功能化 功能化 原子转移自由基聚合 原子转移自由基聚合 天然植物纤维 天然植物纤维 接枝改性 接枝改性
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| GB/T 7714 | 余方兵 , 潘梅华 , 何素萍 et al. 天然植物纤维ATRP改性的研究进展 [J]. | 生物质化学工程 , 2025 , 59 (01) : 61-70 . |
| MLA | 余方兵 et al. "天然植物纤维ATRP改性的研究进展" . | 生物质化学工程 59 . 01 (2025) : 61-70 . |
| APA | 余方兵 , 潘梅华 , 何素萍 , 杨文斌 . 天然植物纤维ATRP改性的研究进展 . | 生物质化学工程 , 2025 , 59 (01) , 61-70 . |
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As a natural and sustainable high-strength material, bamboo has been widely used in modern architectural landscape and other aspects. Bamboo scrimber is a new engineered bamboo material obtained by a process of dissolving, dipping, and layer-by-layer hot pressing. It offers advantages of high strength, scalability, and versatility. However, bamboo is prone to mildew, which significantly limits the durability of engineered scrimber. In this study, bamboo fiber bundles were soaked in zinc acetate solution and then treated by atmospheric plasma. Zinc oxide nanoparticles were in-situ coated on the surface of bamboo through the high-energy reaction of atmospheric plasma, improving the mildew resistance of bamboo scrimber. Meanwhile, atmospheric plasma can effectively improve the wettability of the bamboo surface, allowing for the retention of the bamboo bark and bamboo inner skin those need to be removed in advance due to poor bonding performance in the preparation of bamboo scrimber. After atmospheric plasma treatment, the adhesive solution can better spread and penetrate the bamboo surface, forming a continuous and stable adhesive layer during the hot pressing process. The experimental results showed that bamboo scrimbers gained outstanding mildew resistance after atmospheric plasma treatment, along with a significant improvement in mechanical strength. This method is energy-saving and efficient, enabling pilot-scale and continuous production of bamboo scrimber, and holds great potential for widespread practical application. © 2025, The Authors. All rights reserved.
Keyword ：
Gluing Gluing High energy forming High energy forming Hot pressing Hot pressing Metal castings Metal castings Plasma CVD Plasma CVD Plasma enhanced chemical vapor deposition Plasma enhanced chemical vapor deposition Scale (deposits) Scale (deposits) Zinc Selenide Zinc Selenide
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| GB/T 7714 | Hong, Guolong , Lin, Chengwei , Chen, Linbi et al. High-Strength Anti-Mildew Bamboo Scrimber Prepared by Atmospheric Plasma-Enhanced Deposition of Zinc Acetate Solution [J]. | SSRN , 2025 . |
| MLA | Hong, Guolong et al. "High-Strength Anti-Mildew Bamboo Scrimber Prepared by Atmospheric Plasma-Enhanced Deposition of Zinc Acetate Solution" . | SSRN (2025) . |
| APA | Hong, Guolong , Lin, Chengwei , Chen, Linbi , Mo, Yuhan , Fei, Mingen , Li, Ran et al. High-Strength Anti-Mildew Bamboo Scrimber Prepared by Atmospheric Plasma-Enhanced Deposition of Zinc Acetate Solution . | SSRN , 2025 . |
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Gypsum particleboard is attracting attention in the construction industry due to its excellent properties. However, the traditional raw materials for gypsum particleboard are facing a shortage of supply. In this study, we innovatively utilized bulk solid waste Phosphogypsum and Pennisetum giganteum for the first time to manufacture gypsum particleboard. This approach not only effectively addresses the issue of insufficient supply of traditional raw materials for gypsum particleboard but also provides a new pathway for the resource utilization of phosphogypsum. Through an orthogonal experimental design, we focused on optimizing the gypsum particleboard formulation, concentrating on factors such as density, the ratio of Pennisetum giganteum to gypsum (grass-plaster ratio), the ratio of water to gypsum (water-plaster ratio), and the size of the particles. The study determined that the optimal formulation parameters were a density of 1.2 g/ cm3, a grass-plaster ratio of 0.20, a water-plaster ratio of 0.25, and a particle mesh number of 14. Under these conditions, the gypsum particleboard exhibited excellent performance, characterized by a static flexural strength of 6.5 MPa, a modulus of elasticity of 2010 MPa, an internal bond strength of 0.4 MPa, a 24-hour water-absorption thickness expansion rate of 2.2%, and an equilibrium moisture content of 1.6%, all meeting the American Society for Testing and Materials (ASTM) Standard D1037. These findings indicate that gypsum particleboards made with Pennisetum giganteum and phosphogypsum can perform comparably to those made with conventional materials. Additionally, a performance prediction model was established using Multiple Linear Regression Analysis (MLRA). The analysis revealed a significant linear relationship between the independent and dependent variables in the model, with the Analysis of Variance (ANOVA) significance levels being less than 0.05, demonstrating statistical significance. This result provides a theoretical basis for the future development of high-performance gypsum particleboard.
Keyword ：
Gypsunm particleboard Gypsunm particleboard Multiple linear regression analysis Multiple linear regression analysis Orthogonal analysis Orthogonal analysis Pennisetum giganteum Pennisetum giganteum Phosphogypsum Phosphogypsum
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| GB/T 7714 | Wu, Nengsen , Huang, Bocong , Xie, Jingzhou et al. Optimizing gypsum particleboard properties: An orthogonal analysis of pennisetum giganteum and phosphogypsum composites [J]. | CASE STUDIES IN CONSTRUCTION MATERIALS , 2024 , 20 . |
| MLA | Wu, Nengsen et al. "Optimizing gypsum particleboard properties: An orthogonal analysis of pennisetum giganteum and phosphogypsum composites" . | CASE STUDIES IN CONSTRUCTION MATERIALS 20 (2024) . |
| APA | Wu, Nengsen , Huang, Bocong , Xie, Jingzhou , Huang, Ping , Yang, Wenbin , Xu, Qing . Optimizing gypsum particleboard properties: An orthogonal analysis of pennisetum giganteum and phosphogypsum composites . | CASE STUDIES IN CONSTRUCTION MATERIALS , 2024 , 20 . |
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