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学者姓名：张慧
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Abstract ：
The widespread use of antibiotics in marine aquaculture poses a significant threat to the ecological equilibrium and human health. Collaborative adsorption-photocatalysis based on metal organic framework (MOF) catalysts has emerged as an advanced and highly effective strategy for removing antibiotics from aquatic environments. However, the intrinsic limitations of MOF including their low photocatalytic efficiency and susceptibility to structural collapse hinder their widespread practical application. Inspired by the symbiotic relationship between sea anemones and hermit crabs, we prepared a floating, anisotropic MIL-53 (Fe/Co)-graphene oxide/sodium alginate/nanocellulose composite aerogel (FCG/SC) catalyst via graphene oxide (GO) interface regulation and directional freeze-drying technology for efficient degradation of antibiotics in water. Strategic doping of Co elements within Fe-MOF metal nodes constructed defect structures and improved the catalytic performance. The introduction of GO in the hydrothermal reaction not only facilitates the nucleation of Fe/Co metal cations but also regulates the catalyst particle size and suppresses electron-hole recombination, ultimately enhancing photocatalytic efficiency. Furthermore, the directional channel structure of the aerogel shortens the light path, maximizing light absorption on the catalyst surface. The results indicated that the synergistic adsorptionphotocatalytic (SAP) degradation of tetracycline hydrochloride (TC-HCl) exhibited superior efficiency compared to the pre-adsorption photocatalysis (PAP) processes. A significant SAP efficiency of 99.32 % was achieved when the MIL-53 (Fe/Co)-graphene oxide loading rate reached 30 wt%. Moreover, FCG/SC exhibited exceptional SAP degradation efficiency of 70.12 % even challenged with aquaculture wastewater containing NH4Cl, KNOB, NaNO2, KH2PO4, and glucose. Crucially, the FCG/SC demonstrated exceptional stability and reusability. Five consecutive cycles revealed no substantial damage to the surface structure or catalyst leaching, and the degradation efficiency still can be remained at 96.16 %. This highly efficient and reusable composite aerogel offers a novel approach for the removal of TC-HCl from marine aquaculture wastewater.
Keyword ：
Aerogel Aerogel Antibiotics removal Antibiotics removal Degradation Degradation Metal organic framework Metal organic framework Photocatalytic Photocatalytic
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| GB/T 7714 | Lin, Xiaoxia , Chen, Yongli , Li, Keying et al. A floatable and anisotropic composite aerogel for enhanced synergistic adsorption-catalysis of antibiotics in marine aquaculture wastewater [J]. | DESALINATION , 2026 , 618 . |
| MLA | Lin, Xiaoxia et al. "A floatable and anisotropic composite aerogel for enhanced synergistic adsorption-catalysis of antibiotics in marine aquaculture wastewater" . | DESALINATION 618 (2026) . |
| APA | Lin, Xiaoxia , Chen, Yongli , Li, Keying , Han, Xiyue , Zhang, Xuexia , Li, Yuqi et al. A floatable and anisotropic composite aerogel for enhanced synergistic adsorption-catalysis of antibiotics in marine aquaculture wastewater . | DESALINATION , 2026 , 618 . |
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Multifunctional wearable flexible electronic devices based on hydrogels have received extensive research in recent years. Despite their promising applications, a significant challenge persists in terms of efficiently powering these devices. Triboelectric nanogenerators (TENGs) assembled by surface-modified hydrogels may be one of the promising strategies to address this challenge. This study presents the development of a multifunctional composite hydrogel, which is synthesized through the amino surface modification of glycerin-cellulose hydrogel (3-aminopropyltriethoxysilane-glycerin-cellulose, A-GC). The resulting composite hydrogel is utilized in the fabrication of electrodes of TENGs, which can effectively harvest mechanical energy to power flexible sensors. By using cellulose and glycerin as primary raw materials and 3-aminotriethoxysilane as surface modification components, the composite hydrogel exhibits excellent mechanical properties, coupled with good electrical conductivity (2.83 S/m). More importantly, it exhibits a high triboelectric output performance of 205.3 V, maintains stable long-term triboelectric output, and achieves a maximum triboelectric power density of 732.1 mW/m2. Furthermore, the introduction of glycerin into the cellulose hydrogel enhances its mechanical properties and triboelectric output performance even under extreme environmental conditions (-24 and 60 degrees C). The A-GC-TENG demonstrates significant potential in various applications, including mechanical energy harvesting and conversion, writing recognition, wireless signal transmission, and human-computer interaction, showing great application prospects in flexible wearable sensors and self-powered electronic devices. The development of the composite cellulose hydrogel offers a novel approach for the fabrication of high-performance flexible wearable electronic devices, which is capable of functioning effectively in harsh environments.
Keyword ：
Cellulose hydrogel Cellulose hydrogel Mechanical property Mechanical property Surface modification Surface modification Triboelectric nanogenerator Triboelectric nanogenerator
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| GB/T 7714 | Liu, Afei , Zheng, Siyu , Wu, Wenhui et al. Surface amination modification of cellulose hydrogels for enhancing triboelectric performance of extreme environment-resistant triboelectric sensors [J]. | JOURNAL OF BIORESOURCES AND BIOPRODUCTS , 2026 , 11 (1) . |
| MLA | Liu, Afei et al. "Surface amination modification of cellulose hydrogels for enhancing triboelectric performance of extreme environment-resistant triboelectric sensors" . | JOURNAL OF BIORESOURCES AND BIOPRODUCTS 11 . 1 (2026) . |
| APA | Liu, Afei , Zheng, Siyu , Wu, Wenhui , Liu, Jiaqing , Zhang, Hui , Chen, Lihui et al. Surface amination modification of cellulose hydrogels for enhancing triboelectric performance of extreme environment-resistant triboelectric sensors . | JOURNAL OF BIORESOURCES AND BIOPRODUCTS , 2026 , 11 (1) . |
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Nanofluidic membranes composed of polymers and metal-organic frameworks (MOFs) are considered ideal for efficiently harvesting salinity gradient energy from global estuaries due to their well-defined nanochannels and surface charge. However, developing a polymer/MOF membrane that simultaneously combines excellent mechanical strength, scalability, high surface charge density, and porous structure remains a significant challenge. Here, we demonstrated a hybrid nanofluidic membrane by deconstructing charged cellulosic fibers (CCF) into charged cellulose molecules (CCM) and then tandemly connecting imidazolate molecular sieve framework-8 (ZIF-8). In this regard, the CCM/ZIF-8 nanofluidic membrane inherits a high surface charge density of CCF (-44 mV for zeta potential), abundant-angstrom/nanopore distinction of ZIF-8 (1540.5 m(2)/g for specific surface area and sub-nanometer pore size), and thus demonstrates excellent chemical and structural uniqueness, and superior robustness (similar to 25 MPa), high stability (stable for over 30 days in acidic, alkaline, and seawater environments) and scalability. As a result, our CCM/ZIF-8 membrane enables an excellent cation selectivity (t(+) of 0.82) and correspondingly high power density of up to 8.7 W/m(2) in KCl system (0.01/0.5 M salinity gradient, testing area of 0.075 mm(2)) and stably output over 60 days. This study provides a promising strategy for constructing high-performance polymer/MOF nanofluidic membranes for advanced selective ion transport, beyond salinity gradient energy conversion.
Keyword ：
Biomass Biomass Energy harvesting Energy harvesting Nanofluidic Nanofluidic Robustness Robustness Tandemly connecting Tandemly connecting
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| GB/T 7714 | Shi, Jianping , Zhang, Xinyuan , Wang, Yingchao et al. Robust nanofluidic membrane: Charged cellulose tandem angstrom/ nanochanneled ZIF-8 [J]. | CHEMICAL ENGINEERING JOURNAL , 2025 , 507 . |
| MLA | Shi, Jianping et al. "Robust nanofluidic membrane: Charged cellulose tandem angstrom/ nanochanneled ZIF-8" . | CHEMICAL ENGINEERING JOURNAL 507 (2025) . |
| APA | Shi, Jianping , Zhang, Xinyuan , Wang, Yingchao , Liu, Yiku , Niu, Shengyue , Mondal, Ajoy Kanti et al. Robust nanofluidic membrane: Charged cellulose tandem angstrom/ nanochanneled ZIF-8 . | CHEMICAL ENGINEERING JOURNAL , 2025 , 507 . |
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Flexible hybrid nanogenerators (HNGs) have received significant attention for their potential in harvesting mechanical energy to power portable and miniaturized portable devices. This work presents a method to fabricate flexible, durable and biodegradable electrospun polydopamine@barium titanate/cellulose acetate (PDA@BTO/CA) nanofiber films. This design integrates polydopamine (PDA) and piezoelectric barium titanate (BTO) nanoparticles within a flexible cellulose acetate (CA) matrix to enable self-powered wearable biomonitoring. The inclusion of PDA enhances the physical adhesion between BTO and CA, resulting in a significant 40% increase in voltage output. Notably, the PDA-modified composite PDA@BTO/CA demonstrates remarkable durability over 15,000 cycles and effectively detects a range of human motions (such as fist clenching, wrist bending, elbow movement, walking, running and jumping), transducing them into stable, precise electrical signals. Intriguingly, the hybrid nanogenerator device exhibits robust performance in extreme conditions, including underwater and high or low temperatures, while maintaining its good biodegradability. This work paves the way for advanced self-powered wearable biosensor devices capable of precise and reliable human motion monitoring.
Keyword ：
Cellulose Cellulose Composite Composite Hybrid nanogenerator Hybrid nanogenerator Polydopamine Polydopamine Wearable sensors Wearable sensors
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| GB/T 7714 | Lu, Shengchang , Li, Shuai , Li, Qin et al. Flexible cellulose-based hybrid nanogenerators for self-powered wearable bio-monitoring applications [J]. | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2025 , 685 : 1087-1098 . |
| MLA | Lu, Shengchang et al. "Flexible cellulose-based hybrid nanogenerators for self-powered wearable bio-monitoring applications" . | JOURNAL OF COLLOID AND INTERFACE SCIENCE 685 (2025) : 1087-1098 . |
| APA | Lu, Shengchang , Li, Shuai , Li, Qin , Yang, Lin , Zhang, Hui , Li, Jianguo et al. Flexible cellulose-based hybrid nanogenerators for self-powered wearable bio-monitoring applications . | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2025 , 685 , 1087-1098 . |
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Tetracycline (TC) is a common antibiotic; when untreated TC enters the environment, it will cause a negative impact on the human body through the food chain. In the present study, MnO2/MCM-41@Fe3O4 (FeMnMCM) prepared using a hydrothermal and redox method and Camellia oleifera shell-activated carbon (COFAC) prepared through alkali activation were encapsulated using alginate (ALG) and calcium chloride as a cross-linking matrix to give the composite beads COFAC-FeMnMCM-ALG. The resultant COFAC-FeMnMCM-ALG composite beads were then carefully characterized, showing a high immobilization of MnO2/MCM-41@Fe3O4, with porous COFAC as an effective bioadsorbent for enriching the pollutants in the treated samples. These bead catalysts were subsequently applied to the oxidative degradation of TC in a Fenton oxidation system. Several parameters affecting the degradation were investigated, including the H2O2 concentration, catalyst dosage, initial TC concentration, and temperature. A very high catalytic activity towards the degradation of TC was demonstrated. The electron paramagnetic resonance (EPR) and quenching results showed that OH and O-2(-) were generated in the system, with OH as the main radical species. In addition, the COFAC-FeMnMCM-ALG catalyst exhibited excellent recyclability/reusability. We conclude that the as-prepared COFAC-FeMnMCM-ALG composite beads, which integrate MnO2 and Fe3O4 with bioadsorbents, provide a new idea for the design of catalysts for advanced oxidation processes (AOPs) and have great potential in the Fenton oxidation system to degrade toxic pollutants.
Keyword ：
alginate alginate catalyst catalyst COFAC COFAC composite beads composite beads MnO2/MCM-41@Fe3O4 MnO2/MCM-41@Fe3O4 tetracycline tetracycline
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| GB/T 7714 | Zheng, Zhigong , Shi, Ronghui , Zhang, Xiaoping et al. Preparation of Activated Carbon-Reinforced Composite Beads Based on MnO2/MCM-41@Fe3O4 and Calcium Alginate for Efficient Removal of Tetracycline in Aqueous Solutions [J]. | POLYMERS , 2024 , 16 (8) . |
| MLA | Zheng, Zhigong et al. "Preparation of Activated Carbon-Reinforced Composite Beads Based on MnO2/MCM-41@Fe3O4 and Calcium Alginate for Efficient Removal of Tetracycline in Aqueous Solutions" . | POLYMERS 16 . 8 (2024) . |
| APA | Zheng, Zhigong , Shi, Ronghui , Zhang, Xiaoping , Ni, Yonghao , Zhang, Hui . Preparation of Activated Carbon-Reinforced Composite Beads Based on MnO2/MCM-41@Fe3O4 and Calcium Alginate for Efficient Removal of Tetracycline in Aqueous Solutions . | POLYMERS , 2024 , 16 (8) . |
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Membrane separation technology is a vital method for separating oil/water emulsions. However, membrane fouling caused by repeated use has brought a series of problems such as reduced permeation flux and poor recycling. Herein, we fabricated a high-flux and self-cleaning electrospinning nanofiber membrane Polyacrylonitrile-NH2-MIL-88B(PAN-NH2-M88B) by a facile one-step electrospinning blending method for highly efficient oil/water emulsion separation. Benefit from the constructed micro/nano rough structure and hydrophilic surface of NH2-MIL-88B(NH2-M88B), the PAN-NH2-M88B membrane exhibited excellent separation performances, high wettability and permeation flux after multiple oil/water emulsion separation tests under visible light irradiation. The fabricated nanofiber membrane can achieve a high separation efficiency of 99.5 % and a high flux of 5095-7662 L m(-2)h(-1) respectively for five types of oil-in-water emulsions. More importantly, the flux of the fabricated nanofiber membrane is 2-3 times that of the membrane prepared by the traditional phase conversion method, which greatly reduces the separation time and improves the separation efficiency. Moreover, the flux of the oil-contaminated membrane can be restored by simple visible light irradiation, demonstrating excellent photocatalytic self-cleaning property. Therefore, the membrane has good stability and can be reused for many times with little change in separation efficiency and flux. Owing to the facile preparation method and the excellent performances, the developed nanofiber membrane was expected to be an ideal candidate for industrial oil-water emulsion separation.
Keyword ：
Electrospinning Electrospinning Emulsion separation Emulsion separation High flux High flux Nanofiber membrane Nanofiber membrane Self-cleaning Self-cleaning
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| GB/T 7714 | Lin, Xiaoxia , Li, Bingzhang , Liu, Zongyang et al. High flux, self-cleaning electrospun nanofiber membrane using one-step blending method for highly efficient oil-in-water emulsion separation [J]. | SEPARATION AND PURIFICATION TECHNOLOGY , 2024 , 334 . |
| MLA | Lin, Xiaoxia et al. "High flux, self-cleaning electrospun nanofiber membrane using one-step blending method for highly efficient oil-in-water emulsion separation" . | SEPARATION AND PURIFICATION TECHNOLOGY 334 (2024) . |
| APA | Lin, Xiaoxia , Li, Bingzhang , Liu, Zongyang , Yin, Hao , Zheng, Chenghui , Li, Yuqi et al. High flux, self-cleaning electrospun nanofiber membrane using one-step blending method for highly efficient oil-in-water emulsion separation . | SEPARATION AND PURIFICATION TECHNOLOGY , 2024 , 334 . |
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Breathable membranes with micropores enable the transfer of gas molecules while blocking liquids and solids, and have a wide range of applications in medical, industrial, environmental, and energy fields. Breathability is highly influenced by the nature of a material, pore size, and pore structure. Preparation methods and the incorporation of functional materials are responsible for the variety of physical properties and applications of breathable membranes. In this review, the preparation methods of breathable membranes, including blown film extrusion, cast film extrusion, phase separation, and electrospinning, are discussed. According to the antibacterial, hydrophobic, thermal insulation, conductive, and adsorption properties, the application of breathable membranes in the fields of electronics, medicine, textiles, packaging, energy, and the environment are summarized. Perspectives on the development trends and challenges of breathable membranes are discussed.
Keyword ：
application application breathable breathable electrospinning electrospinning hydrophobic hydrophobic membrane membrane micropore micropore
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| GB/T 7714 | Luo, Tingshuai , Farooq, Ambar , Weng, Wenwei et al. Progress in the Preparation and Application of Breathable Membranes [J]. | POLYMERS , 2024 , 16 (12) . |
| MLA | Luo, Tingshuai et al. "Progress in the Preparation and Application of Breathable Membranes" . | POLYMERS 16 . 12 (2024) . |
| APA | Luo, Tingshuai , Farooq, Ambar , Weng, Wenwei , Lu, Shengchang , Luo, Gai , Zhang, Hui et al. Progress in the Preparation and Application of Breathable Membranes . | POLYMERS , 2024 , 16 (12) . |
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Abstract ：
人才是新质生产力的第一资源。为着力培养材料与化工领域高层次、应用型专门人才，深入探索并创新了产教融合的人才培养新路径：强化思想价值引领，构建双导师协同育人体系，打造高质量实践基地，完善专业实践考核与保障机制，以及建立毕业生跟踪反馈与评价机制。这一系列举措旨在全方位、多维度地优化人才培养模式，为提高材料与化工专业学位研究生创新实践能力提供坚实支撑与有效策略，进而为行业输送更多具备实战能力和创新思维的高端人才。
Keyword ：
专业学位 专业学位 产教融合 产教融合 教学改革 教学改革 新质生产力 新质生产力 材料与化工 材料与化工
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| GB/T 7714 | 周吓星 , 余雁 , 陈奶荣 et al. 产教融合协同育人，赋能新质生产力发展——以福建农林大学材料与化工专业学位研究生培养为例 [J]. | 纸和造纸 , 2024 , 43 (05) : 10-13 . |
| MLA | 周吓星 et al. "产教融合协同育人，赋能新质生产力发展——以福建农林大学材料与化工专业学位研究生培养为例" . | 纸和造纸 43 . 05 (2024) : 10-13 . |
| APA | 周吓星 , 余雁 , 陈奶荣 , 罗小林 , 张慧 , 陈礼辉 . 产教融合协同育人，赋能新质生产力发展——以福建农林大学材料与化工专业学位研究生培养为例 . | 纸和造纸 , 2024 , 43 (05) , 10-13 . |
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Photocatalytic water treatment is an advanced and efficient technology for water purification. Among various photocatalysts, iron-based metal-organic frameworks (Fe-MOFs) are widely applied for mineralizing organic wastewater due to their excellent water stability and photocatalytic activity. However, their practical application is impeded by insufficient photocatalytic performance, irreversible collapse of the framework structure during repeated use, and difficulty in recovery. In this study, we fabricated a Graphene oxide (GO) structure-oriented NH2-MIL-88B(Fe)/graphene oxide/sodium alginate (NM88B/GO/SA) aerogel for the removal of dyes and antibiotics, using GO interface regulation and dual-network crosslinking methods. In this hybrid system, a NM88B/GO heterostructure was formed through the directional growth of NM88B on the surface of GO. The introduction of sodium alginate (SA) enhanced the robustness and stability of the matrix, and effectively avoided aerogel fragmentation. With 30 wt% catalyst loading, the composite aerogel exhibited excellent photocatalytic degradation performance towards high-concentration (50 ppm) tetracycline hydrochloride (TC-HCl), achieving over 99% removal rate in 150 min. It also effectively degraded methylene blue (MB) at 10-30 ppm with over 99% removal rate. Furthermore, the aerogel showed excellent shape recovery ability, stability, and reusability. After five repeated tests, it maintained over 95% degradation efficiency for both TC-HCl and MB. This advanced aerogel holds great promise as a highly efficient and reusable photocatalyst for removing antibiotics and dyes from wastewater.
Keyword ：
Aerogel Aerogel Degradation Degradation Metal-organic frameworks Metal-organic frameworks Photocatalytic Photocatalytic Recyclability Recyclability
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| GB/T 7714 | Lin, Xiaoxia , Zhao, Jie , Zhang, Yongqi et al. Graphene Oxide Structure-Oriented NM88B/GO/SA Aerogel for Highly Efficient Degradation of Dye and Antibiotic Wastewater [J]. | JOURNAL OF POLYMERS AND THE ENVIRONMENT , 2023 , 32 (5) : 2091-2104 . |
| MLA | Lin, Xiaoxia et al. "Graphene Oxide Structure-Oriented NM88B/GO/SA Aerogel for Highly Efficient Degradation of Dye and Antibiotic Wastewater" . | JOURNAL OF POLYMERS AND THE ENVIRONMENT 32 . 5 (2023) : 2091-2104 . |
| APA | Lin, Xiaoxia , Zhao, Jie , Zhang, Yongqi , Li, Yuqi , Liao, Yiqiang , Zhang, Hui . Graphene Oxide Structure-Oriented NM88B/GO/SA Aerogel for Highly Efficient Degradation of Dye and Antibiotic Wastewater . | JOURNAL OF POLYMERS AND THE ENVIRONMENT , 2023 , 32 (5) , 2091-2104 . |
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Numerous materials with special wetting properties have been achieved for oil spillage cleanup. However, most of them need complicated fabrication procedure or involve expensive or toxic chemicals, leading to high production cost and secondary pollution. In the present study, a robust, cost–effective and hydrophobic nanofibrillated cellulose (NFC)/ chitosan (CS) aerogel was developed using a convenient dip-coating technique, followed by a solution–aerogel conversion strategy. To achieve hydrophobic property, the low–cost stearic acid (SA) was used as a modifier instead of the traditional expensive silane coupling agents. The stearic acid modified chitosan/ nanofibrillated cellulose (SA–NFC/CS) aerogel exhibited high oil absorption capacities, 76.8 g g−1 for kerosene and 142.5 g g−1 for chloroform. More importantly, the hydrophobic aerogel could be repeatedly used through a simple mechanical squeezing process. All these features make the SA–NFC/CS aerogel a promising candidate for the effective and targeted removal of oily contaminants from wastewater. © 2023, The Authors. All rights reserved.
Keyword ：
Aerogels Aerogels Cellulose Cellulose Chitosan Chitosan Chlorine compounds Chlorine compounds Costs Costs Coupling agents Coupling agents Hydrophobicity Hydrophobicity Organic pollutants Organic pollutants Stearic acid Stearic acid Water absorption Water absorption Water pollution Water pollution Water treatment Water treatment
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| GB/T 7714 | Ni, Shuzhen , Li, Yuqi , Han, Wenjia et al. Green Approach to Prepare Hydrophobic Nanofibrillated Cellulose/Chitosan Aerogel for the Effective Removal of Oily Pollutants from Water [J]. | SSRN , 2023 . |
| MLA | Ni, Shuzhen et al. "Green Approach to Prepare Hydrophobic Nanofibrillated Cellulose/Chitosan Aerogel for the Effective Removal of Oily Pollutants from Water" . | SSRN (2023) . |
| APA | Ni, Shuzhen , Li, Yuqi , Han, Wenjia , Zhang, Hui , Shi, Ronghui . Green Approach to Prepare Hydrophobic Nanofibrillated Cellulose/Chitosan Aerogel for the Effective Removal of Oily Pollutants from Water . | SSRN , 2023 . |
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