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学者姓名：廖光福
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Abstract ：
Metal organic framework (MOF)-based photocatalysts for solar-driven fuel generation have seen significant advancement owing to their structural and porous controllability, high surface area, and distinctive semiconductor property. In this review, the opto-electronic characteristics of MOF-based photocatalysts are firstly introduced. After that, the fabrication strategies for MOF-based photocatalysts are illustrated. Then, some typical MOF-based photocatalysts for energy-related applications are exhibited. Lastly, this review also offers some indepth perceptions into significant difficulties, advantageous situations, and heuristic possibilities for future improvement. There is no question that the newly developed MOF-based photocatalysts can achieve new innovations for energy-related applications.
Keyword ：
Metal organic frameworks Metal organic frameworks Opto-electronic properties Opto-electronic properties Photocatalysis Photocatalysis Solar-driven fuel production Solar-driven fuel production Synthesis methods Synthesis methods
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| GB/T 7714 | Li, Chunxue , Huang, Ning-Yu , Yang, Yingkui et al. Emerging metal-organic framework-based photocatalysts for solar-driven fuel production [J]. | COORDINATION CHEMISTRY REVIEWS , 2025 , 524 . |
| MLA | Li, Chunxue et al. "Emerging metal-organic framework-based photocatalysts for solar-driven fuel production" . | COORDINATION CHEMISTRY REVIEWS 524 (2025) . |
| APA | Li, Chunxue , Huang, Ning-Yu , Yang, Yingkui , Xu, Qiang , Liao, Guangfu . Emerging metal-organic framework-based photocatalysts for solar-driven fuel production . | COORDINATION CHEMISTRY REVIEWS , 2025 , 524 . |
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Electrocatalytic oxidation of inexpensive 5-hydroxymethylfurfural (HMF) into valuable chemicals (e.g., 2,5-furancarboxylic acid (FDCA)) is an inevitable trend in the real-world applications. Nevertheless, it is still difficult to create durable, highly effective, and selective electrocatalysts with enough oxidation current density. Herein, a sulfur (S)-doped nickel-iron layered double hydroxide (S-NiFe LDH) electrocatalyst was successfully fabricated through co-precipitation and hydrothermal strategies, which showcase the effectively catalyze the oxidation reaction of HMF (HMFOR) at a low overpotential (1.36 V vs RHE) with a high current density (20 mA cm-2), displaying excellent stability and 97.3 % FDCA selectivity. It has been discovered that S doping can modify the HMFOR reaction pathway and promote the production of the S-NiOOH active species. Furthermore, the findings of theoretical calculations show that S doping raises the electrical interaction between active species and HMF and lowers the adsorption energy of HMF. With its novel use of doped LDH catalysts for HMFOR, this work offers a hopeful view on energy transformation and the electrocatalytic machining of monomers produced from biomass.
Keyword ：
5-Hydroxymethylfurfural 5-Hydroxymethylfurfural Electrocatalytic oxidation reaction Electrocatalytic oxidation reaction Layered double hydroxides Layered double hydroxides Sulfur doping Sulfur doping
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| GB/T 7714 | Zhang, Juntao , Yang, Yong , Ding, Guixiang et al. Electrooxidation of biomass-derived 5-hydroxymethylfurfural over sulfur-doped nickel-iron layered double hydroxides nanosheets [J]. | CHEMICAL ENGINEERING JOURNAL , 2025 , 505 . |
| MLA | Zhang, Juntao et al. "Electrooxidation of biomass-derived 5-hydroxymethylfurfural over sulfur-doped nickel-iron layered double hydroxides nanosheets" . | CHEMICAL ENGINEERING JOURNAL 505 (2025) . |
| APA | Zhang, Juntao , Yang, Yong , Ding, Guixiang , Wang, Zhaoqiang , Wang, Peng , Li, Chunuxe et al. Electrooxidation of biomass-derived 5-hydroxymethylfurfural over sulfur-doped nickel-iron layered double hydroxides nanosheets . | CHEMICAL ENGINEERING JOURNAL , 2025 , 505 . |
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Photocatalytic CO2 reduction into high-value C2+ products such as C2H6 is of great importance but challenging due to their multi-electron steps and high energy barrier of C & horbar;C coupling. Moreover, improving its solar-to-chemical (STC) energy conversion efficiency in pure water beyond the current 1% empirical value is also a significant challenge. Herein, graphite carbon nitride (g-C3N4) nanosheets with controllable carbon (C) doping and nitrogen (N) vacancies (PCCN-x) are designed through a biochar-tailored protocol for efficiently and selectively photo-converting CO2 into C2H6. The optimal PCCN-10 photocatalyst enables the achievement of an exceptional C2H6 activity of 99.14 mu mol g(-1) h(-1) with C2H6 selectivity of 80.33% over 20 h in pure water. A record STC efficiency of approximate to 1.13% for solar fuel production from CO2 and H2O vapor is also achieved without any other energy inputs. Outdoor tests also demonstrated an impressive CO2-to-C2H6 photo-conversion rate of 43.17 mu mol g(-1) h(-1) in pure water, with stable activity over 50 h period. Critically, experimental and theoretical calculations further confirm the pivotal role of bridged C sites and N vacancies in activating CO2 molecules and promoting the formation of C & horbar;C coupling intermediate (*OCCO), which is very beneficial for the production of C2H6. The impressive performance of this work in the photocatalytic conversion of CO2 to high-value C2H6 fuels paves the way for large-scale fuel production and broader sustainable applications.
Keyword ：
C2H6 C2H6 carbon doping carbon doping carbon nitride carbon nitride C & horbar;C coupling C & horbar;C coupling nitrogen vacancies nitrogen vacancies
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| GB/T 7714 | Chen, Zihe , Ding, Guixiang , Wang, Zhaoqiang et al. Precision Molecular Engineering of Carbon Nitride for Efficient and Selective Photoreduction of CO2 to C2H6 in Pure Water [J]. | ADVANCED FUNCTIONAL MATERIALS , 2025 , 35 (25) . |
| MLA | Chen, Zihe et al. "Precision Molecular Engineering of Carbon Nitride for Efficient and Selective Photoreduction of CO2 to C2H6 in Pure Water" . | ADVANCED FUNCTIONAL MATERIALS 35 . 25 (2025) . |
| APA | Chen, Zihe , Ding, Guixiang , Wang, Zhaoqiang , Xiao, Yin , Liu, Xin , Chen, Lihui et al. Precision Molecular Engineering of Carbon Nitride for Efficient and Selective Photoreduction of CO2 to C2H6 in Pure Water . | ADVANCED FUNCTIONAL MATERIALS , 2025 , 35 (25) . |
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Hydrogels made of plant-derived biomass have gained popularity in biomedical applications because they are frequently affordable, readily available, and biocompatible. Finding the perfect plant-derived biomass-based hydrogels for biomedicine that can replicate essential characteristics of human tissues in regard to structure, function, and performance has proved to be difficult. In this review, we summarize some of the major contributions made to this topic, covering basic ideas and different biomass-based hydrogels made of cellulose, hemicellulose, and lignin. Also included is an in-depth discussion regarding the biosafety and toxicity assessments of biomass-based hydrogels. Finally, this review also highlights important scientific debates and major obstacles regarding biomass based hydrogels for biomedical applications.
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| GB/T 7714 | Li, Tushuai , Sun, Wenxue , Qian, Da et al. Plant-derived biomass-based hydrogels for biomedical applications [J]. | TRENDS IN BIOTECHNOLOGY , 2025 , 43 (4) : 802-811 . |
| MLA | Li, Tushuai et al. "Plant-derived biomass-based hydrogels for biomedical applications" . | TRENDS IN BIOTECHNOLOGY 43 . 4 (2025) : 802-811 . |
| APA | Li, Tushuai , Sun, Wenxue , Qian, Da , Wang, Peng , Liu, Xingyu , He, Chengsheng et al. Plant-derived biomass-based hydrogels for biomedical applications . | TRENDS IN BIOTECHNOLOGY , 2025 , 43 (4) , 802-811 . |
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The valorization of carbon dioxide into high-value-added hydrocarbons, especially light olefins (C2-C4=) through sustainable energy input holds significant industrial value, offering a route for producing essential chemical feedstocks while simultaneously mitigating the emission of this potent greenhouse gas. Despite significant advancements in CO2 hydrogenation technologies, developing efficient catalysts capable of effectively managing C-O bond activation and facilitating C-C bond growth with high conversion rates and desired selectivity for low-carbon olefins, remains a significant challenge. This high-caliber review explores the transformative potential of CO2 valorization into C2-C4=, offering an innovative pathway to produce vital chemical feedstocks while addressing greenhouse gas emissions. Focusing on the CO2-modified Fischer-Tropsch synthesis through iron- catalyst, recognized for its energy efficiency and suitability for C2-C4= production through thermocatalytic CO2 hydrogenation. Key highlights include in-depth analyses of the dynamic nature of catalytically active iron phases, novel materials, and state-of-the-art catalyst design strategies to overcome the challenges of Anderson-Schulz- Flory (ASF) limitations and low olefin selectivity. With a comprehensive discussion on reaction mechanisms, catalyst composition, and performance-driving factors, this review sets the stage for pioneering advancements in catalyst development. Thus, by bridging fundamental insights with cutting-edge technologies, this work provides strategic guidance for developing the next generation of efficient and sustainable catalytic systems for CO2 hydrogenation.
Keyword ：
CO 2 hydrogenation CO 2 hydrogenation Fischer-Tropsch synthesis process Fischer-Tropsch synthesis process Iron-based catalysts Iron-based catalysts Light olefins Light olefins Thermocatalysis Thermocatalysis
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| GB/T 7714 | Liu, Kun , Nawaz, Muhammad Asif , Liao, Guangfu . Decoding fundamental insights and outlooks on state-of-the-art iron-catalyst design strategies for meliorated CO2 valorization into light olefins [J]. | COORDINATION CHEMISTRY REVIEWS , 2025 , 535 . |
| MLA | Liu, Kun et al. "Decoding fundamental insights and outlooks on state-of-the-art iron-catalyst design strategies for meliorated CO2 valorization into light olefins" . | COORDINATION CHEMISTRY REVIEWS 535 (2025) . |
| APA | Liu, Kun , Nawaz, Muhammad Asif , Liao, Guangfu . Decoding fundamental insights and outlooks on state-of-the-art iron-catalyst design strategies for meliorated CO2 valorization into light olefins . | COORDINATION CHEMISTRY REVIEWS , 2025 , 535 . |
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One of the primary challenges for immune checkpoint blockade (ICB)-based therapy is the limited infiltration of T lymphocytes (T cells) into tumors, often referred to as immunologically "cold" tumors. A promising strategy to enhance the anti-tumor efficacy of ICB is to increase antigen exposure, thereby enhancing T cell activation and converting "cold" tumors into "hot" ones. Herein, we present an innovative all-in-one therapeutic nanoplatform to realize local mild photothermal- and photodynamic-triggered antigen exposure, thereby improving the anti-tumor efficacy of ICB. This nanoplatform involves conjugating programmed death-ligand 1 antibody (aPD-L1) with gadolinium-doped near-infrared (NIR)-emitting carbon dots (aPD-L1@GdCDs), which displays negligible cytotoxicity in the absence of light. But under controlled NIR laser irradiation, the GdCDs produce combined photothermal and photodynamic effects. This not only results in tumor ablation but also induces immunogenic cell death (ICD), facilitating enhanced infiltration of CD8(+) T cells in the tumor area. Importantly, the combination of aPD-L1 with photothermal and photodynamic therapies via aPD-L1@GdCDs significantly boosts CD8(+) T cell infiltration, reduces tumor size, and improves anti-metastasis effects compared to either GdCDs-based phototherapy or aPD-L1 alone. In addition, the whole treatment process can be monitored by multi-modal fluorescence/photoacoustic/magnetic resonance imaging (FLI/PAI/MRI). Our study highlights a promising nanoplatform for cancer diagnosis and therapy, as well as paves the way to promote the efficacy of ICB therapy through mild photothermal- and photodynamic-triggered immunotherapy.
Keyword ：
Immune checkpoint blockade Immune checkpoint blockade Immunogenic cell death Immunogenic cell death Multi-modal imaging Multi-modal imaging Photo-immunotherapy Photo-immunotherapy Red emissive carbon dots Red emissive carbon dots
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| GB/T 7714 | Fan, Yadi , Zhang, Ruolin , Shi, Jingyu et al. Mild near-infrared laser-triggered photo-immunotherapy potentiates immune checkpoint blockade via an all-in-one theranostic nanoplatform [J]. | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2025 , 678 : 1088-1103 . |
| MLA | Fan, Yadi et al. "Mild near-infrared laser-triggered photo-immunotherapy potentiates immune checkpoint blockade via an all-in-one theranostic nanoplatform" . | JOURNAL OF COLLOID AND INTERFACE SCIENCE 678 (2025) : 1088-1103 . |
| APA | Fan, Yadi , Zhang, Ruolin , Shi, Jingyu , Tian, Feng , Zhang, Yu , Zhang, Li et al. Mild near-infrared laser-triggered photo-immunotherapy potentiates immune checkpoint blockade via an all-in-one theranostic nanoplatform . | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2025 , 678 , 1088-1103 . |
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Piezo-photocatalysis is capable of concerting mechanical vibration into chemical energy, portraying a promising alternative technology for H2O2 production. However, low mechanical energy conversion efficiency and constrained surface active sites hinder its practical application. Herein, ultrathin porous carbon nitride nanosheets with controlled carbon vacancies and oxygen doping (OCN-X, where X represents the calcination temperature) are synthesized by thermal oxidation etching to achieve unprecedented piezo-photocatalytic H2O2 production. The carbon vacancies and oxygen doping cause the formation of asymmetric structure of triazine unit with a strong dipole field, which creates spontaneous polarization field to speed up directional electron transfer to the nitrogen active sites for effective piezo-photocatalysis. Meanwhile, the ultrathin and porous structure formed by hot-oxygen etching enhances the mechanical energy conversion efficiency and collaboratively induces adsorbed oxygen via indirect two-electron oxygen reduction reaction (ORR) transfer pathway to effectively produce H2O2. Consequently, without any co-catalysts, the as-prepared OCN-460 displays record-high piezo-photocatalytic H2O2 production rate of 19.30 mmol g-1 h-1, far outdistancing those previously reported for piezo-photocatalysts. Furthermore, it also still maintains a notable piezo-photocatalytic activity of 2.87 mmol g-1 h-1 in the pure water system. This work offers some new insights for the future design of an effective piezo-photocatalytic H2O2 production system.
Keyword ：
Defective carbon nitride Defective carbon nitride Dipole field Dipole field Piezo-photocatalysis Piezo-photocatalysis Ultrathin nanosheets Ultrathin nanosheets
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| GB/T 7714 | Wang, Zhaoqiang , Ding, Guixiang , Huang, Hongwei et al. Unraveling the dipole field in ultrathin, porous, and defective carbon nitride nanosheets for record-high piezo-photocatalytic H2O2 production [J]. | ESCIENCE , 2025 , 5 (3) . |
| MLA | Wang, Zhaoqiang et al. "Unraveling the dipole field in ultrathin, porous, and defective carbon nitride nanosheets for record-high piezo-photocatalytic H2O2 production" . | ESCIENCE 5 . 3 (2025) . |
| APA | Wang, Zhaoqiang , Ding, Guixiang , Huang, Hongwei , Zhang, Juntao , Lv, Qi , Shuai, Li et al. Unraveling the dipole field in ultrathin, porous, and defective carbon nitride nanosheets for record-high piezo-photocatalytic H2O2 production . | ESCIENCE , 2025 , 5 (3) . |
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The unique benefits of nickel-aluminium layered double hydroxide (Ni-Al LDH)-based heterojunctions, including large surface area, tunable bandgap and morphology, abundant reaction sites, and high activity, selectivity, and photostability, make them extremely promising for photocatalytic applications. Given the importance and benefits of Ni-Al LDH-based heterojunctions in photocatalysis, it is necessary to provide a summary of Ni-Al LDH-based heterojunctions for photocatalytic applications. Hence, in this review, we thoroughly described the material design for Ni-Al LDH-based heterojunctions, along with their recent developments in various photocatalytic applications, i.e., H2 evolution, CO2 reduction, and pollutant removal. Moreover, the most recent advancements, difficulties, and future prospects of Ni-Al LDH-based heterojunctions for photocatalytic applications were emphasized and thoroughly examined. Undoubtedly, in the near future, scientific researchers will put relentless efforts to exploit new Ni-Al LDH-based heterojunctions for high-performance photocatalytic applications.
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| GB/T 7714 | Li, Chunxue , Ding, Guixiang , Wang, Peng et al. Emerging frontiers of nickel-aluminium layered double hydroxide heterojunctions for photocatalysis [J]. | DALTON TRANSACTIONS , 2025 , 54 (3) : 889-897 . |
| MLA | Li, Chunxue et al. "Emerging frontiers of nickel-aluminium layered double hydroxide heterojunctions for photocatalysis" . | DALTON TRANSACTIONS 54 . 3 (2025) : 889-897 . |
| APA | Li, Chunxue , Ding, Guixiang , Wang, Peng , Liu, Kun , Yang, Bin , Liao, Guangfu . Emerging frontiers of nickel-aluminium layered double hydroxide heterojunctions for photocatalysis . | DALTON TRANSACTIONS , 2025 , 54 (3) , 889-897 . |
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The piezo-photocatalysis enhanced by piezoelectric nanogenerators is considered one of the most effective methods for treating emerging contaminants (ECs) in environmental water. In this study, BiFeO3/ZnIn2S4/Ag (BFO/ZIS/Ag) with boosting piezo-photocatalytic performance was synthesized by modulating the interaction between the step-scheme (S-scheme) heterojunction and the Mott-Schottky barrier. The catalytic rate of the optimized BFO/ZIS/Ag-0.01 catalyst is 4.85 x 10-2 min- 1 for the degradation of niazitidine (NZT) under both ultrasonic and visible light radiation, which is respectively 4.3 and 4.8 times higher than that of pure BFO and ZIS. Furthermore, the total organic carbon (TOC) test revealed that NZT degradation reached 98.4 % after 120 min of continuous reaction. This enhanced piezo-photocatalytic performance is mainly due to the synergistic effect of integrated heterojunction and piezoelectric field. DFT calculations revealed that the charge transfer enhancement at the heterogeneous interface resulted from directional electron transfer to ZIS via Zn-O and S-Ag channels, following the introduction of Ag nanoparticles, which shortened the carrier separation path. Additionally, BFO bent the band of the composite catalyst, promoting carrier separation. These resulted in the generation of abundant highly active 1O2, which specifically targeted and disrupted stable NZT molecules. Moreover, BFO/ZIS/Ag-0.01 exhibited strong inhibitory and antibacterial effects against Escherichia coli and Staphylococcus aureus via electrostatic adsorption and ionization. This study offers new insights into the restoration of aquatic environments and bacterial disinfection through the use of piezoelectric catalytic materials.
Keyword ：
Charge separation Charge separation Hollow nanosphere Hollow nanosphere Piezo-photocatalytic Piezo-photocatalytic
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| GB/T 7714 | Liu, Sheng , Zhang, Yanjun , Guo, Yujuan et al. Step-scheme/Mott-Schottky integrated heteroiunctions in BiFeO3/ZnIn2S4/ Ag hollow nanospheres: Facilitating efficient piezo-photocatalytic activation of peroxydisulfate to enhance nizatidine degradation and antibacterial activity [J]. | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2025 , 686 : 45-62 . |
| MLA | Liu, Sheng et al. "Step-scheme/Mott-Schottky integrated heteroiunctions in BiFeO3/ZnIn2S4/ Ag hollow nanospheres: Facilitating efficient piezo-photocatalytic activation of peroxydisulfate to enhance nizatidine degradation and antibacterial activity" . | JOURNAL OF COLLOID AND INTERFACE SCIENCE 686 (2025) : 45-62 . |
| APA | Liu, Sheng , Zhang, Yanjun , Guo, Yujuan , Cheng, Zhenping , Yuan, Mengyi , Xu, Zushun et al. Step-scheme/Mott-Schottky integrated heteroiunctions in BiFeO3/ZnIn2S4/ Ag hollow nanospheres: Facilitating efficient piezo-photocatalytic activation of peroxydisulfate to enhance nizatidine degradation and antibacterial activity . | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2025 , 686 , 45-62 . |
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Photocatalytic peroxydisulfate (PDS) activation is considered as a promising strategy for antibiotic degradation due to it possesses abundant active species, but the activation effect is limited by low redox capacity and carrier separation efficiency. Herein, a Zn0.5Cd0.5S/g-C3N4 (ZCS/g-C3N4) S-scheme heterojunction with high carrier separation efficiency is synthesized for the degradation of ciprofloxacin (CIP). The reaction rate constant of 1:2 ZCS/g-C3N4 + PDS (0.0461 min-1 ) is approximately 4.43 times and 5.36 times that of ZCS + PDS (0.0104 min-and g-C3N4 + PDS (0.0086 min-1 ). In addition to comparable photocatalytic activity, the photocatalyst also shows good chemical stability, which can be attributed to that the S-scheme heterojunction inhibits the photocorrosion behavior of ZCS. Based on in-situ X-ray photoelectron spectroscopy (XPS), theoretical calculation, and photoassisted Kelvin probe force microscopy (KPFM) results, S-scheme electron migration pathway is proposed. The constructed S-scheme heterojunction with the properties of "One Stone and Two Birds", which solve two important problems simultaneously including low carrier migration rate and severe photocorrosion. Finally, the constructed photocatalyst possesses comparable catalytic activity and excellent chemical stability. This study proves the practicality of 1:2 ZCS/g-C3N4 + PDS for CIP degradation, which provides a theoretical basis for further research on water environmental remediation.
Keyword ：
Ciprofloxacin Ciprofloxacin Photocatalytic peroxydisulfate activation Photocatalytic peroxydisulfate activation Photocorrosion behavior Photocorrosion behavior S-scheme heterojunction S-scheme heterojunction
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| GB/T 7714 | Li, Chunxue , Cheng, Bohan , Shen, Jyunhong et al. Photocatalytic peroxydisulfate activation over Zn0.5Cd0.5S/g-C3N4 S-scheme heterojunction: " One Stone and two Birds" strategy to improve the photocatalytic activity and stability [J]. | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 360 . |
| MLA | Li, Chunxue et al. "Photocatalytic peroxydisulfate activation over Zn0.5Cd0.5S/g-C3N4 S-scheme heterojunction: " One Stone and two Birds" strategy to improve the photocatalytic activity and stability" . | SEPARATION AND PURIFICATION TECHNOLOGY 360 (2025) . |
| APA | Li, Chunxue , Cheng, Bohan , Shen, Jyunhong , Wang, Haoshuai , Yi, Mingxiu , Gu, Panyang et al. Photocatalytic peroxydisulfate activation over Zn0.5Cd0.5S/g-C3N4 S-scheme heterojunction: " One Stone and two Birds" strategy to improve the photocatalytic activity and stability . | SEPARATION AND PURIFICATION TECHNOLOGY , 2025 , 360 . |
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