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学者姓名：林冠烽
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Abstract ：
Tetracycline (TC) and its derivatives pose a serious threat to the ecological environment and human health due to their high toxicity and difficult degradation, and there is an urgent need to develop an effective degradation technology for their efficient removal. In this study, FeP/phosphorus-doped carbon aerogel (FeP/PCA) with dual advantages of degradation and adsorption was constructed by a one-step synthesis strategy using sodium carboxymethyl cellulose (CMC) as a carbon source, phytic acid as a phosphorus source, and ferric chloride as an iron source, and was applied as an advanced oxidation catalyst for the removal of TC. Under the combined effect of adsorption, in situ oxygen activation and electron transfer, FeP/PCA achieved 100 % removal and 72.9 % mineralization of TC. Desorption and Ar pre-blowing experiments showed that the contributions of FeP/PCA to the adsorption, in situ oxygen activation, and electron transfer were 53.2 %, 28.0 %, and 18.8 %, respectively. FeP/PCA adsorbed dissolved oxygen (DO) from water and induced in-situ oxygen activation through FeP and carbon substrate defects, which drove the Fenton-like reaction to generate reactive oxygen species (center dot O2-, center dot OH, and 1 O 2 ) to efficiently degrade TC. Among them, center dot O 2 - provides a primary role. In addition, FeP induced changes in the electronic structure of PCA, leading to electron transfer of sp2 C--C, sp3 C-C, C-O/C-P and C--O, resulting in a synergistic degradation effect. This study presents for the first time a novel composite material with both adsorption and catalytic degradation advantages that can be used for the practical treatment of antibiotic wastewater.
Keyword ：
FeP/PCA FeP/PCA Iron-based catalysts Iron-based catalysts Phosphorus doping Phosphorus doping Reactive oxygen species Reactive oxygen species Tetracycline Tetracycline
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| GB/T 7714 | Wang, Guilong , Jiang, Rongyuan , Chen, Juntao et al. One-step construction of FeP/carbon aerogel composites and their efficient tetracycline removal mechanisms: Adsorption, in situ oxygen activation and electron transfer [J]. | JOURNAL OF WATER PROCESS ENGINEERING , 2025 , 70 . |
| MLA | Wang, Guilong et al. "One-step construction of FeP/carbon aerogel composites and their efficient tetracycline removal mechanisms: Adsorption, in situ oxygen activation and electron transfer" . | JOURNAL OF WATER PROCESS ENGINEERING 70 (2025) . |
| APA | Wang, Guilong , Jiang, Rongyuan , Chen, Juntao , Li, Simin , Lin, Guanfeng , Lu, Beili et al. One-step construction of FeP/carbon aerogel composites and their efficient tetracycline removal mechanisms: Adsorption, in situ oxygen activation and electron transfer . | JOURNAL OF WATER PROCESS ENGINEERING , 2025 , 70 . |
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本发明公开了一种环氧大豆油‑木质素‑多元酸三元胶黏剂及其制备方法和应用，其是将木质素、多元醇和水混合后进行机械研磨，然后将研磨产物与环氧大豆油、多元酸/酸酐和溶剂混合搅拌或研磨，从而得到所述三元胶黏剂。本发明充分利用了木质素和环氧大豆油的天然优势，通过简化的制备方法，提高了胶黏剂的整体性能，解决了传统石油基胶黏剂存在有害物质释放，而生物基胶黏剂在高湿度或高温环境下性能稳定性受限的问题。该胶黏剂可广泛应用于胶合板、纤维板、刨花板、竹木复合板等领域，具有优异的环保性能和工业应用性能。
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| GB/T 7714 | 刘瀚杨 , 黄彪 , 卢贝丽 et al. 一种环氧大豆油-木质素-多元酸三元胶黏剂及制备方法 : CN202410265557.1[P]. | 2024-03-08 . |
| MLA | 刘瀚杨 et al. "一种环氧大豆油-木质素-多元酸三元胶黏剂及制备方法" : CN202410265557.1. | 2024-03-08 . |
| APA | 刘瀚杨 , 黄彪 , 卢贝丽 , 唐丽荣 , 吕建华 , 游昕达 et al. 一种环氧大豆油-木质素-多元酸三元胶黏剂及制备方法 : CN202410265557.1. | 2024-03-08 . |
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Phosphorus-doped hard carbon/MnOx composites were synthesized by hydrothermal treatment and one-step pyrolysis using coconut shell as a biomass carbon source, phosphoric acid as a phosphorus source and a pore-forming agent, and manganese sulphate as a manganese source, and were used in the field of supercapacitors. The effects of the additions of phosphoric acid and manganese sulfate on the structural and electrochemical properties of the composites were analyzed, and the mechanism of the enhancement of the electrochemical properties of phosphorus-doped hard carbon/MnOx composites was investigated. The etching of phosphoric acid contributed to the formation of a multistage pore structure of microporous-mesoporous composite, which provided not only the composites with bilayer capacitance, but also space for the growth of MnOx and reduced its agglomeration, thus exposing more pseudocapacitive active sites. Phosphorus doping not only increased the layer spacing of the hard carbon and improved the defects in its structure, but also introduced phosphorus-containing functional groups such as C-P==O, C-P-O and C/P-O-P, which synergistically interacted with MnOx to further enhance its electrochemical performance. The specific capacitance of the composite was as high as 302F/g, and the capacitance retention was still 70.5% after 10000 cycles at 10A/g. When assembled into a symmetric supercapacitor, the power density was up to 400W/kg at the energy density of 156Wh/kg, which indicated that it had a great potential for application in the field of supercapacitors. © 2025 Chemical Industry Press Co., Ltd.. All rights reserved.
Keyword ：
Capacitance Capacitance Doping (additives) Doping (additives) Electrochemical properties Electrochemical properties Manganese compounds Manganese compounds Microporosity Microporosity Phosphorus Phosphorus Pore structure Pore structure Porous carbon Porous carbon Sulfur compounds Sulfur compounds Supercapacitor Supercapacitor
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| GB/T 7714 | Jiang, Rongyuan , Li, Simin , Chen, Zhiqiang et al. Preparation of phosphorus-doped hard carbon/MnOx composite and its electrochemical properties [J]. | Chemical Industry and Engineering Progress , 2025 , 44 (7) : 4039-4049 . |
| MLA | Jiang, Rongyuan et al. "Preparation of phosphorus-doped hard carbon/MnOx composite and its electrochemical properties" . | Chemical Industry and Engineering Progress 44 . 7 (2025) : 4039-4049 . |
| APA | Jiang, Rongyuan , Li, Simin , Chen, Zhiqiang , Wang, Guilong , Chen, Juntao , Lin, Guanfeng et al. Preparation of phosphorus-doped hard carbon/MnOx composite and its electrochemical properties . | Chemical Industry and Engineering Progress , 2025 , 44 (7) , 4039-4049 . |
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Cellulose acetate (CA), a biomass-derived material for desalination membranes, faces challenges in nanofiltration-based desalination due to its weakly charged hydroxyl groups. Here we report gradient-charged CA membranes (GC-CAMs) engineered through the surface segregation of ionic covalent organic framework nanosheets (iCOFNs). Pre-evaporation drives sulfonated iCOFNs to migrate from the bulk to the surface due to the density difference between the nanosheets and CA solution, which creates a gradient distribution of iCOFNs and forms GC-CAMs via phase inversion. The charged nanosheets enriched on the front surface increase the membrane charge density from -0.89 to -1.13 mC m(-2) while decreasing membrane pore size from 0.74 to 0.68 nm, synergistically enhancing ion exclusion via electrostatic repulsion and size sieving. By positioning the front membrane surface downstream, salt rejection is further improved by mitigating the charge shielding effect. By regulating the pre-evaporation time and iCOFN content, the optimized GC-CAM achieves a Na2SO4 rejection of similar to 95 %, which is maintained at similar to 90 % over two months. When applied to natural water purification, it reduces total dissolved solids by similar to 83 % while moderately removing heavy metal ions. The proposed gradient structure offers a novel approach for the charge engineering of nanofiltration membranes.
Keyword ：
Cellulose acetate membrane Cellulose acetate membrane Gradient-charged distribution Gradient-charged distribution Ionic covalent organic framework Ionic covalent organic framework Nanofiltration-based desalination Nanofiltration-based desalination Surface segregation Surface segregation
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| GB/T 7714 | Chen, Ran , Luo, Shan , Song, Zifan et al. Gradient-charged cellulose acetate membranes enabled by ionic COF nanosheets for enhanced nanofiltration-based desalination [J]. | JOURNAL OF MEMBRANE SCIENCE , 2025 , 734 . |
| MLA | Chen, Ran et al. "Gradient-charged cellulose acetate membranes enabled by ionic COF nanosheets for enhanced nanofiltration-based desalination" . | JOURNAL OF MEMBRANE SCIENCE 734 (2025) . |
| APA | Chen, Ran , Luo, Shan , Song, Zifan , Tian, Youqing , Shi, Dai , Lu, Beili et al. Gradient-charged cellulose acetate membranes enabled by ionic COF nanosheets for enhanced nanofiltration-based desalination . | JOURNAL OF MEMBRANE SCIENCE , 2025 , 734 . |
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用超临界二氧化碳萃取技术（SFE）提取杉木精油，并以提取精油后的杉木屑残渣为原料，利用磷酸活化法制备高吸附木质活性炭，对萃取条件及磷酸浸渍工艺进行优化，得到SFE萃取杉木精油的较佳条件为萃取温度35℃、萃取压力30 MPa、萃取时间100 min,该条件下杉木精油得率达2.42%。磷酸浸渍的较佳工艺条件为浸渍温度130℃、浸渍时间60 min,磷酸质量分数55%,该条件下制备的活性炭，其碘吸附值达865.8 mg/g,亚甲基蓝吸附值达285.0 mg/g,能满足商业应用要求。采用SEM、BET以及XRD表征杉木萃取精油前后的形貌特征、孔隙结构以及纤维素结晶区结构演变，并探究SFE对萃取后杉木屑的磷酸浸渍工艺影响。结果表明：SFE在精油提取过程中使杉木屑表面生成一定孔隙，杉木屑萃取精油后，其比表面积从2.04 m
Keyword ：
二氧化碳超临界 二氧化碳超临界 杉木精油 杉木精油 活性炭 活性炭 联产技术 联产技术
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| GB/T 7714 | 文世涛 , 卢辛成 , 徐茹婷 et al. 杉木屑提取精油及制活性炭联产技术研究 [J]. | 林产化学与工业 , 2025 , 45 (03) : 113-120 . |
| MLA | 文世涛 et al. "杉木屑提取精油及制活性炭联产技术研究" . | 林产化学与工业 45 . 03 (2025) : 113-120 . |
| APA | 文世涛 , 卢辛成 , 徐茹婷 , 许伟 , 林冠烽 , 孙康 . 杉木屑提取精油及制活性炭联产技术研究 . | 林产化学与工业 , 2025 , 45 (03) , 113-120 . |
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目的 解决单一组分壳聚糖成膜性能不佳，无法满足食品包装商业应用需求的问题。综述壳聚糖基保鲜膜/涂层应用于食品包装领域的可能性。方法 对现有文献进行系统梳理并综合分析，介绍壳聚糖基保鲜膜/涂层的多样化制备技术、改性策略及性能表征，并概述壳聚糖基保鲜膜/涂层在食品包装领域最新的应用研究进展。结论 通过对壳聚糖进行物理/化学改性，可以显著改善其光学、力学、阻隔和抗菌等方面的性能。最后对壳聚糖基保鲜膜/涂层在食品包装领域的应用潜力进行了展望，指出了未来研究的重点方向。
Keyword ：
保鲜膜/涂层 保鲜膜/涂层 壳聚糖 壳聚糖 改性策略 改性策略
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| GB/T 7714 | 沈永康 , 朱峰 , 冯雪锋 et al. 壳聚糖基保鲜膜/涂层的制备及应用 [J]. | 包装工程 , 2025 , 46 (01) : 79-88 . |
| MLA | 沈永康 et al. "壳聚糖基保鲜膜/涂层的制备及应用" . | 包装工程 46 . 01 (2025) : 79-88 . |
| APA | 沈永康 , 朱峰 , 冯雪锋 , 崔钰圆 , 黄明堦 , 林冠烽 et al. 壳聚糖基保鲜膜/涂层的制备及应用 . | 包装工程 , 2025 , 46 (01) , 79-88 . |
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以椰壳为生物质碳源，磷酸为磷源和造孔剂，硫酸锰为锰源，通过水热处理和一步热解法合成磷掺杂硬碳/MnO
Keyword ：
MnO MnO 椰壳 椰壳 磷掺杂 磷掺杂
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| GB/T 7714 | 江荣源 , 李思敏 , 陈志强 et al. 磷掺杂硬碳/MnO [J]. | 化工进展 , 2025 , 44 (07) : 4039-4049 . |
| MLA | 江荣源 et al. "磷掺杂硬碳/MnO" . | 化工进展 44 . 07 (2025) : 4039-4049 . |
| APA | 江荣源 , 李思敏 , 陈志强 , 王贵龙 , 陈俊涛 , 林冠烽 et al. 磷掺杂硬碳/MnO . | 化工进展 , 2025 , 44 (07) , 4039-4049 . |
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本发明公开了一种竹木基生物环氧胶黏剂的制备方法及其应用，其是通过将竹/木原料粉碎并磨粉后，将所得粉体与多元醇和水混合并静置，之后通过机械研磨实现竹粉、木粉的微纳化；再将其与环氧化合物、多元酸/酸酐和溶剂混合，经搅拌反应制得所述竹木基生物环氧胶黏剂。本发明利用丰富的竹木资源，创新性地开发了一种全新的胶黏剂，其具有优异的粘接强度、耐水性、耐热性以及良好的环境友好性，可直接应用于通过热压实现固化粘合的领域，如制备胶合板、纤维板、刨花板、竹木复合板等，以应对传统石油基胶黏剂的环境和健康问题，同时克服了现有生物基胶黏剂在粘接性能方面的不足。
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| GB/T 7714 | 黄彪 , 刘瀚杨 , 唐丽荣 et al. 一种竹木基生物环氧胶黏剂的制备方法和应用 : CN202410265523.2[P]. | 2024-03-08 . |
| MLA | 黄彪 et al. "一种竹木基生物环氧胶黏剂的制备方法和应用" : CN202410265523.2. | 2024-03-08 . |
| APA | 黄彪 , 刘瀚杨 , 唐丽荣 , 卢贝丽 , 吕建华 , 游昕达 et al. 一种竹木基生物环氧胶黏剂的制备方法和应用 : CN202410265523.2. | 2024-03-08 . |
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以椰壳为生物质碳源，磷酸为磷源和造孔剂，硫酸锰为锰源，通过水热处理和一步热解法合成磷掺杂硬碳/MnO
Keyword ：
MnO MnO 椰壳 椰壳 磷掺杂 磷掺杂
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| GB/T 7714 | 江荣源 , 李思敏 , 陈志强 et al. 磷掺杂硬碳/MnO x 复合材料的制备及其电化学性能 [J]. | 化工进展 , 2025 , 44 (07) : 4039-4049 . |
| MLA | 江荣源 et al. "磷掺杂硬碳/MnO x 复合材料的制备及其电化学性能" . | 化工进展 44 . 07 (2025) : 4039-4049 . |
| APA | 江荣源 , 李思敏 , 陈志强 , 王贵龙 , 陈俊涛 , 林冠烽 et al. 磷掺杂硬碳/MnO x 复合材料的制备及其电化学性能 . | 化工进展 , 2025 , 44 (07) , 4039-4049 . |
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生物质基碳材料因其在储能领域的潜力受到了广泛关注。然而，纯碳基材料通常亲水性差、赝电容低；组装成电极时需要使用黏结剂，限制了其在高能量密度超级电容器上的应用。基于此，本研究以植酸为造孔剂和磷源，制备出自支撑磷掺杂厚碳电极（P-WC），并将其应用于超级电容器中。植酸的造孔和掺杂作用赋予P-WC三维多孔结构和超亲水性，这促进了电解液快速渗透和交换，显著提升其电化学性能。组装成对称超级电容器（SSC）时，在1mA/cm
Keyword ：
厚碳电极 厚碳电极 杨木 杨木 植酸 植酸 磷掺杂 磷掺杂 超级电容器 超级电容器
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| GB/T 7714 | 李思敏 , 江荣源 , 陈志强 et al. 自支撑掺磷厚碳电极的构建及其在超级电容器中的应用 [J]. | 化工进展 , 2025 , 44 (11) : 6258-6269 . |
| MLA | 李思敏 et al. "自支撑掺磷厚碳电极的构建及其在超级电容器中的应用" . | 化工进展 44 . 11 (2025) : 6258-6269 . |
| APA | 李思敏 , 江荣源 , 陈志强 , 袁春雯 , 王贵龙 , 陈俊涛 et al. 自支撑掺磷厚碳电极的构建及其在超级电容器中的应用 . | 化工进展 , 2025 , 44 (11) , 6258-6269 . |
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