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学者姓名：陈礼辉
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Abstract ：
Multifunctional wearable flexible electronic devices based on hydrogels have received extensive research in recent years. Despite their promising applications, a significant challenge persists in terms of efficiently powering these devices. Triboelectric nanogenerators (TENGs) assembled by surface-modified hydrogels may be one of the promising strategies to address this challenge. This study presents the development of a multifunctional composite hydrogel, which is synthesized through the amino surface modification of glycerin-cellulose hydrogel (3-aminopropyltriethoxysilane-glycerin-cellulose, A-GC). The resulting composite hydrogel is utilized in the fabrication of electrodes of TENGs, which can effectively harvest mechanical energy to power flexible sensors. By using cellulose and glycerin as primary raw materials and 3-aminotriethoxysilane as surface modification components, the composite hydrogel exhibits excellent mechanical properties, coupled with good electrical conductivity (2.83 S/m). More importantly, it exhibits a high triboelectric output performance of 205.3 V, maintains stable long-term triboelectric output, and achieves a maximum triboelectric power density of 732.1 mW/m2. Furthermore, the introduction of glycerin into the cellulose hydrogel enhances its mechanical properties and triboelectric output performance even under extreme environmental conditions (-24 and 60 degrees C). The A-GC-TENG demonstrates significant potential in various applications, including mechanical energy harvesting and conversion, writing recognition, wireless signal transmission, and human-computer interaction, showing great application prospects in flexible wearable sensors and self-powered electronic devices. The development of the composite cellulose hydrogel offers a novel approach for the fabrication of high-performance flexible wearable electronic devices, which is capable of functioning effectively in harsh environments.
Keyword ：
Cellulose hydrogel Cellulose hydrogel Mechanical property Mechanical property Surface modification Surface modification Triboelectric nanogenerator Triboelectric nanogenerator
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| GB/T 7714 | Liu, Afei , Zheng, Siyu , Wu, Wenhui et al. Surface amination modification of cellulose hydrogels for enhancing triboelectric performance of extreme environment-resistant triboelectric sensors [J]. | JOURNAL OF BIORESOURCES AND BIOPRODUCTS , 2026 , 11 (1) . |
| MLA | Liu, Afei et al. "Surface amination modification of cellulose hydrogels for enhancing triboelectric performance of extreme environment-resistant triboelectric sensors" . | JOURNAL OF BIORESOURCES AND BIOPRODUCTS 11 . 1 (2026) . |
| APA | Liu, Afei , Zheng, Siyu , Wu, Wenhui , Liu, Jiaqing , Zhang, Hui , Chen, Lihui et al. Surface amination modification of cellulose hydrogels for enhancing triboelectric performance of extreme environment-resistant triboelectric sensors . | JOURNAL OF BIORESOURCES AND BIOPRODUCTS , 2026 , 11 (1) . |
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Abstract ：
Wearable sensing electronic devices based on hydrogel are gradually developing towards multifunction and portability, however, efficiently harvesting energy from the surrounding environment to power traditional hydrogel-based wearable electronic devices is a major challenge. The assembly of multilayer heterogeneous hydrogels is a potential strategy to address this challenge. Herein, inspired by the structure of diodes, a diode-like integrated hydrogel composed of a three-tier structure of anionic polyelectrolyte hydrogel, polyacrylamide hydrogel and cationic polyelectrolyte hydrogel is developed. By the connection of polyacrylamide hydrogel, the composite hydrogel exhibits excellent structural stability and mechanical properties. Notably, due to the introduction of MXene ion-conducting microchannels, the directional transport of free cations and anions ionized by anionic and cationic polyelectrolytes is achieved, thereby improving the conductivity (74.58 mS/cm), sensing (gauge factor = 7.47) and piezoionic output performance of the composite hydrogel. The composite hydrogelbased sensor can sense tiny facial movements and recognize the direction of human movement, and the composite hydrogel-based piezoionic generator exhibit more efficient mechanical-electric conversion performance, which can output the maximum voltage of 1410 mV, current of 28 mu A, and power density of 2.9 mW/m2 for a composite hydrogel of 5x5 cm2. The integration of multilayer heterogeneous hydrogels proposes a versatile strategy for the development of high-performance hydrogel-based self-powered sensing electronic devices, expanding the application of hydrogels in artificial intelligence and human-computer interaction.
Keyword ：
Diode-like Diode-like Hydrogel Hydrogel MXene MXene Piezoionic generator Piezoionic generator Sensor Sensor
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| GB/T 7714 | Zheng, Siyu , Liu, Afei , Liu, Jiaqing et al. A diode-like integrated hydrogel for piezoionic generators and sensors [J]. | NANO ENERGY , 2025 , 133 . |
| MLA | Zheng, Siyu et al. "A diode-like integrated hydrogel for piezoionic generators and sensors" . | NANO ENERGY 133 (2025) . |
| APA | Zheng, Siyu , Liu, Afei , Liu, Jiaqing , Wu, Wenhui , Zhou, Xiaxing , Chen, Lihui et al. A diode-like integrated hydrogel for piezoionic generators and sensors . | NANO ENERGY , 2025 , 133 . |
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Adhesive patches are optimum candidates for distinct biomedical applications, including tissue adhesion and leakage sealing in outpatient or surgical procedures. Unfortunately, most adhesive patches are significantly less effective at providing strong adhesion to the surface of wet tissue, which increases the risk and reduces the fault tolerance in surgery. Meanwhile, customization is difficult to achieve in terms of mechanical adaptability. To tackle this problem, we developed a chitosan-containing bioadhesive patch (ANC) comprising dual-crosslinked carboxymethyl chitosan methacrylate (CMCS-MA), acrylic acid, and acrylic acid N-hydroxysuccinimide ester. This ingenious and convenient design strategy facilitates the integrated polymerization of the patch, while circumventing the necessity for additional crosslinkers. ANC patches in dry state and the rich carboxyl groups contained therein enable rapid removal of moisture from tissue surfaces. Subsequently, robust adhesion based on hydrogen bonding and N-hydroxysuccinimide (NHS)-amine interaction is formed. The dual-crosslinked ANC patch achieves good adjustable mechanical performance and swelling behavior by controlling the addition of CMCS-MA. Furthermore, compared with commercially available fibrin glue, ANC patches own robust adhesion and superior sealing performance for stomach fluid leakage. This intricately designed ANC patch sheds new light on biomedical patch design and broadens the scope of chitosan-containing materials in tissue adhesive and sealant applications.
Keyword ：
adhesive adhesive chitosan chitosan dual-crosslinked dual-crosslinked patch patch
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| GB/T 7714 | Yang, Jiayu , Li, Qiaoling , Zhang, Jianpeng et al. A Chitosan-Containing Dual-Crosslinked Resilient Patch for Tissue Adhesive and Sealant [J]. | CHEMISTRY & BIODIVERSITY , 2025 , 22 (9) . |
| MLA | Yang, Jiayu et al. "A Chitosan-Containing Dual-Crosslinked Resilient Patch for Tissue Adhesive and Sealant" . | CHEMISTRY & BIODIVERSITY 22 . 9 (2025) . |
| APA | Yang, Jiayu , Li, Qiaoling , Zhang, Jianpeng , Wu, Siyang , Zhang, Min , Chen, Lihui et al. A Chitosan-Containing Dual-Crosslinked Resilient Patch for Tissue Adhesive and Sealant . | CHEMISTRY & BIODIVERSITY , 2025 , 22 (9) . |
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Cellulose-based hydrogels are promising materials for constructing flexible supercapacitors and energy storage devices due to their environmental sustainability and resource renewability. However, preparing cellulose-based hydrogel electrolytes with super flexibility, high conductivity, and high specific capacitance for practical applications is still challenging. Herein, an adhesive, antibacterial, conductive zwitterionic cellulose nanofibersreinforced poly(sulfobetaine methacrylate-acrylic acid-acrylamide (ZCNF/PSAA) composite hydrogel was fabricated by a blue light-triggered free radical polymerization of 2-methacryloyloxy ethyl dimethyl-3sulfopropyl ammonium hydroxide (SBMA), acrylic acid (AA), acryl amide (AM), dopamine methacrylamide (DMA) and zwitterionic cellulose nanofibers (ZCNF). The prepared hydrogel exhibited excellent mechanical properties with tensile strength of 0.17 MPa, compressive strength of 0.87 MPa, and shear strength of 1.25 MPa, respectively. The zwitterionic groups significantly enhanced the hydrogel's conductivity (5.8 S/m). Moreover, the hydrogel with electrically sensitive perception of external strain (GF = 2.5), can withstand large bending and compression deformations and can be used as a motion sensor to monitor human movements such as arm and finger bending, pressing, and subtle fist clenching. The resulting hydrogel presented excellent antibacterial activity against Escherichia coli and Staphylococcus aureus. As the hydrogel was applied as electrolyte, the developed super-capacitor exhibited a desirable specific capacitance of 404.5 mF.cm-2, with a maximum energy density of 53.93 Wh.kg-1 and capacitance retention of 80.3 % after 2000 consecutive charge-discharge cycles. The ZCNF/ PSAA hydrogel has great potential for applications in flexible strain sensors and energy storage devices.
Keyword ：
Cellulose nanofibers Cellulose nanofibers Electrolytes Electrolytes Hydrogels Hydrogels Sensors Sensors Super-capacitors Super-capacitors Zwitterions Zwitterions
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| GB/T 7714 | Farooq, Ambar , Wanyan, Hongying , Li, Qin et al. An adhesive, antibacterial, conductive zwitterionic cellulose nanofibers-containing hydrogel for flexible strain sensors and super-capacitors [J]. | CARBOHYDRATE POLYMERS , 2025 , 358 . |
| MLA | Farooq, Ambar et al. "An adhesive, antibacterial, conductive zwitterionic cellulose nanofibers-containing hydrogel for flexible strain sensors and super-capacitors" . | CARBOHYDRATE POLYMERS 358 (2025) . |
| APA | Farooq, Ambar , Wanyan, Hongying , Li, Qin , Lu, Shengchang , Huang, Weiqi , Waqas, Muhammad et al. An adhesive, antibacterial, conductive zwitterionic cellulose nanofibers-containing hydrogel for flexible strain sensors and super-capacitors . | CARBOHYDRATE POLYMERS , 2025 , 358 . |
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The in-situ generation of hydrogen peroxide (H2O2) from oxygen and water with semiconductor photocatalysts under illumination is considered as a promising synthesis pathway. However, photocarrier recombination as well as slow transfer of charges involved in carbon nitride (C3N5, CN), are the enduring challenge for photocatalytic activity. Herein, we develop a pi-stacked CN-based composites (CNv-A) coupling natural polyphenolic anthocyanins (A) with defective carbon nitride (CNv) for efficient visible-light-driven H2O2 production. The strengthening pi-stacking (CNv-A) leads to extended electronic transmission networks via effective intermolecular pi-pi interactions, resulting in a high H2O2 generation rate of 147.2 mu mol.L-1.h-1, as well as 42 times that of the pristine CN. The combination of experimental results and theoretical calculations reveals that with the incorporation of anthocyanins, the intermolecular pi-pi stacking reconstructs the enlarged charge transfer networks over carbon nitride, thus facilitating electron transfer and active center dot O2- generation. Moreover, increasing the content of nitrogen vacancy of carbon nitride effectively strengthened the pi-pi interactions, accelerating the transfer and separation of charge carriers, thereby achieving drastic high-performance H2O2 production via an indirect single-electron oxygen reduction reaction (ORR) pathway. This work provides a new perspective for regulating charge transfer and separation by modulating the strength of intermolecular weak interactions.
Keyword ：
Anthocyanins Anthocyanins Carbon nitride Carbon nitride Charge transfer Charge transfer pi-pi stacking pi-pi stacking Vacancy engineering Vacancy engineering
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| GB/T 7714 | Wu, Shengye , Li, Yixi , Wei, Shuaichong et al. Coupling of anthocyanins at defective carbon nitride (C3N5) with π-π stacking for efficient photocatalytic H2O2 generation [J]. | CHEMICAL ENGINEERING JOURNAL , 2025 , 508 . |
| MLA | Wu, Shengye et al. "Coupling of anthocyanins at defective carbon nitride (C3N5) with π-π stacking for efficient photocatalytic H2O2 generation" . | CHEMICAL ENGINEERING JOURNAL 508 (2025) . |
| APA | Wu, Shengye , Li, Yixi , Wei, Shuaichong , Li, Jiashu , Zhang, Fengshan , Li, Jingde et al. Coupling of anthocyanins at defective carbon nitride (C3N5) with π-π stacking for efficient photocatalytic H2O2 generation . | CHEMICAL ENGINEERING JOURNAL , 2025 , 508 . |
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Hydrogen peroxide (H2O2) photosynthesis from oxygen and water has become an attracting route due to its green, low-carbon and sustainable features. Although carbon nitride (CN) is a remarkable semiconductor for photocatalytic H2O2 production, CN also suffers from slow transfer and poor separation efficiency of photogenerated charges due to the intrinsically molecular structures. Herein, we report a facile method to enhance H2O2 evolution with asymmetric CN via molten-salt assisted supramolecular assemblies of melamine and 2,4,6triaminopyrimidine (T). The optimum M-CNT exhibited a photocatalytic H2O2 production rate of 44.63 mu mol center dot L- 1h- 1, which is more than 4 times higher than that of pristine CN without any sacrificial agents. Experimental and DFT results demonstrate T molecule can tune the charge location of CN frameworks, promoting electron transfer and efficient separation. Furthermore, under the synergy of molten salt, the uneven distribution of intramolecular charges can be exacerbated to boost the photocatalytic performance through significant polarization effects. This work provided a paradigm of charge characteristics of carbon nitride via asymmetric molecular engineering for enhanced photocatalytic H2O2 generation.
Keyword ：
Asymmetric structure Asymmetric structure Carbon nitride Carbon nitride Hydrogen peroxide Hydrogen peroxide Photosynthesis Photosynthesis Polarization effect Polarization effect
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| GB/T 7714 | Li, Jiashu , Li, Yixi , Wei, Shuaichong et al. Asymmetric framework engineering of carbon nitride nanotubes for polarization promoted H2O2 photosynthesis [J]. | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY , 2025 , 366 . |
| MLA | Li, Jiashu et al. "Asymmetric framework engineering of carbon nitride nanotubes for polarization promoted H2O2 photosynthesis" . | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY 366 (2025) . |
| APA | Li, Jiashu , Li, Yixi , Wei, Shuaichong , Wu, Shengye , Peng, Zhangyan , Zhang, Fengshan et al. Asymmetric framework engineering of carbon nitride nanotubes for polarization promoted H2O2 photosynthesis . | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY , 2025 , 366 . |
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In this study, cellulose acetate (CA)-based polyamide (PA) nanofiltration membranes (CA-NF-2/0.4) with enhanced antifouling and separation performance were prepared through the interfacial polymerization of diethylenetriamine (DETA) and 1,3,5-benzenetricarbonyl chloride (TMC) for the effective removal of dyes and salt ions. Benefiting from the three reaction sites (primary and secondary amino groups) of DETA, a PA layer with a three-dimensional network structure formed on the CA substrate, imparting the CA-NF-2/0.4 membranes with a strong negative charge (-24.8 mV at pH 7) and a defect-free morphological feature. Consequently, the CA-NF-2/0.4 membranes exhibited high removal efficiencies for various dyes (99% for Rose Bengal and Congo Red, 95.5% for Methyl Orange, and 96.1% for Methylene Blue), as well as various monovalent and divalent salts, including MgCl2 (84.2%), Na2SO4 (92.7%), MgSO4 (91.8%), and NaCl (54.1%). Additionally, the CA-NF-2/0.4 membranes demonstrated excellent antifouling properties [the flux recovery ratio (flux recovery rate > 98.5%), long-term durability, and stability under high operational pressures and salt concentrations] due to their good hydrophilicity (water contact angle of 39.8 degrees) and the hydrogen bonding interaction between the active amine groups of DETA and the -OH groups of the CA support layer. This study presents an effective method for fabricating cellulose-based NF membranes with high separation and antifouling performance, offering insights into the high-value utilization of cellulose-based materials.
Keyword ：
antifouling antifouling cellulose acetate cellulose acetate diethylene triamine diethylene triamine nanofiltration membranes nanofiltration membranes three-dimensionalnetwork structure three-dimensionalnetwork structure
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| GB/T 7714 | Lin, Yaling , Mo, Minfu , Lin, Junkang et al. Cellulose Acetate-Based Polyamide Nanofiltration Membranes by Diethylenetriamine-Assisted Interfacial Polymerization for Effective Removal of Dyes and Salt Ions [J]. | ACS APPLIED POLYMER MATERIALS , 2025 , 7 (7) : 4153-4165 . |
| MLA | Lin, Yaling et al. "Cellulose Acetate-Based Polyamide Nanofiltration Membranes by Diethylenetriamine-Assisted Interfacial Polymerization for Effective Removal of Dyes and Salt Ions" . | ACS APPLIED POLYMER MATERIALS 7 . 7 (2025) : 4153-4165 . |
| APA | Lin, Yaling , Mo, Minfu , Lin, Junkang , Ma, Xiaojuan , Hong, Yubin , Chen, Lihui et al. Cellulose Acetate-Based Polyamide Nanofiltration Membranes by Diethylenetriamine-Assisted Interfacial Polymerization for Effective Removal of Dyes and Salt Ions . | ACS APPLIED POLYMER MATERIALS , 2025 , 7 (7) , 4153-4165 . |
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Photocatalytic CO2 reduction into high-value C2+ products such as C2H6 is of great importance but challenging due to their multi-electron steps and high energy barrier of C & horbar;C coupling. Moreover, improving its solar-to-chemical (STC) energy conversion efficiency in pure water beyond the current 1% empirical value is also a significant challenge. Herein, graphite carbon nitride (g-C3N4) nanosheets with controllable carbon (C) doping and nitrogen (N) vacancies (PCCN-x) are designed through a biochar-tailored protocol for efficiently and selectively photo-converting CO2 into C2H6. The optimal PCCN-10 photocatalyst enables the achievement of an exceptional C2H6 activity of 99.14 mu mol g(-1) h(-1) with C2H6 selectivity of 80.33% over 20 h in pure water. A record STC efficiency of approximate to 1.13% for solar fuel production from CO2 and H2O vapor is also achieved without any other energy inputs. Outdoor tests also demonstrated an impressive CO2-to-C2H6 photo-conversion rate of 43.17 mu mol g(-1) h(-1) in pure water, with stable activity over 50 h period. Critically, experimental and theoretical calculations further confirm the pivotal role of bridged C sites and N vacancies in activating CO2 molecules and promoting the formation of C & horbar;C coupling intermediate (*OCCO), which is very beneficial for the production of C2H6. The impressive performance of this work in the photocatalytic conversion of CO2 to high-value C2H6 fuels paves the way for large-scale fuel production and broader sustainable applications.
Keyword ：
C2H6 C2H6 carbon doping carbon doping carbon nitride carbon nitride C & horbar;C coupling C & horbar;C coupling nitrogen vacancies nitrogen vacancies
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| GB/T 7714 | Chen, Zihe , Ding, Guixiang , Wang, Zhaoqiang et al. Precision Molecular Engineering of Carbon Nitride for Efficient and Selective Photoreduction of CO2 to C2H6 in Pure Water [J]. | ADVANCED FUNCTIONAL MATERIALS , 2025 , 35 (25) . |
| MLA | Chen, Zihe et al. "Precision Molecular Engineering of Carbon Nitride for Efficient and Selective Photoreduction of CO2 to C2H6 in Pure Water" . | ADVANCED FUNCTIONAL MATERIALS 35 . 25 (2025) . |
| APA | Chen, Zihe , Ding, Guixiang , Wang, Zhaoqiang , Xiao, Yin , Liu, Xin , Chen, Lihui et al. Precision Molecular Engineering of Carbon Nitride for Efficient and Selective Photoreduction of CO2 to C2H6 in Pure Water . | ADVANCED FUNCTIONAL MATERIALS , 2025 , 35 (25) . |
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Batteries have become an integral part of today's life and are presented as the most appropriate approach for energy storage; however, the environmental impacts of their vast usage need to be considered. Therefore, it is essential to incorporate eco-friendly materials to design batteries. Cellulose, the most abundant natural polymer, comprises excellent physical, mechanical, and chemical properties. It presents a broad group of functional materials ranging from macro to nanoscale composites that exhibit their potential in energy-related fields. This review provides a comprehensive summary of structural features, the influence of cellulose-based materials on electrochemical performance, and potential applications of cellulose derivatives as separators, electrolytes, binders, and electrodes in advanced energy storage devices, including sodium-ion, zinc-ion, lithium-ion, and lithium-sulfur batteries and gives an insight of the effects of derivatization on application and electrochemical performance of batteries. This review aims to comprehensively understand the vast applications of cellulose derivatives as vital parts of batteries. At last, an outlook of the current issues and future challenges for applications of cellulose-based materials in batteries is presented.
Keyword ：
Batteries Batteries Binders Binders Cellulose Cellulose Electrode Electrode Electrolyte Electrolyte Separator Separator
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| GB/T 7714 | Farooq, Ambar , Wanyan, Hongying , Lu, Shengchang et al. A review on cellulose-based derivatives and composites for sustainable rechargeable batteries [J]. | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES , 2025 , 308 . |
| MLA | Farooq, Ambar et al. "A review on cellulose-based derivatives and composites for sustainable rechargeable batteries" . | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES 308 (2025) . |
| APA | Farooq, Ambar , Wanyan, Hongying , Lu, Shengchang , Mosisa, Mentgistu Tadesse , Zhou, Xiaxing , Xiao, He et al. A review on cellulose-based derivatives and composites for sustainable rechargeable batteries . | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES , 2025 , 308 . |
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The advancement of ecofriendly and high-performance energy transformation systems has driven the development of advanced membrane materials for alkaline water electrolysis (AWE), which conduct hydroxide ions and block the interpenetration of hydrogen and oxygen. The wettability and inadequate gas blocking remain challenges for the AWE membrane. In this study, a hydrophilic polyphenylene sulfide/cellulose/polyphenylene sulfide (PPS/C/PPS) composite membrane with high bubble point pressure (BPP), outstanding oxygen purity, and low area resistance (AR) was fabricated. The porous PPS/C/PPS membrane exhibits a high BPP of 12.4 bar and low AR of 0.014 Omegacm2. Notably, gas purity tests reveal that the oxygen purity is about 99.974%, which is much higher than that of commercial hydrophilic polyphenylene sulfide (C-HPPS) (98.5%). The AWE cell with the PPS/C/PPS composite membrane shows a current density (CD) of 319.2 mAcm-2 in 30 wt % KOH solution at 80 degrees C at a voltage of 2 V, surpassing that of C-HPPS (208.0 mAcm-2). Additionally, the AWE cell exhibits high stability of more than 450 h at KOH solution (30 wt %) without attenuation, emphasizing the membrane's competitive edge and its vast application potential.
Keyword ：
alkaline water electrolysis alkaline water electrolysis bubble point pressure bubble point pressure cellulose cellulose membrane membrane polyphenylene sulfide polyphenylene sulfide
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| GB/T 7714 | Huang, Jianhua , Zheng, Yulian , Wu, Hui et al. Hydrophilic Polyphenylene Sulfide/Cellulose/Polyphenylene Sulfide Composite Membrane with High Bubble Point Pressure and High Oxygen Purity for Alkaline Water Electrolysis [J]. | ACS APPLIED POLYMER MATERIALS , 2025 , 7 (7) : 4322-4328 . |
| MLA | Huang, Jianhua et al. "Hydrophilic Polyphenylene Sulfide/Cellulose/Polyphenylene Sulfide Composite Membrane with High Bubble Point Pressure and High Oxygen Purity for Alkaline Water Electrolysis" . | ACS APPLIED POLYMER MATERIALS 7 . 7 (2025) : 4322-4328 . |
| APA | Huang, Jianhua , Zheng, Yulian , Wu, Hui , Lin, Hui , Hong, Yubin , Chen, Lihui et al. Hydrophilic Polyphenylene Sulfide/Cellulose/Polyphenylene Sulfide Composite Membrane with High Bubble Point Pressure and High Oxygen Purity for Alkaline Water Electrolysis . | ACS APPLIED POLYMER MATERIALS , 2025 , 7 (7) , 4322-4328 . |
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