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学者姓名：黄六莲
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Abstract ：
Cellulose-based hydrogels are promising materials for constructing flexible supercapacitors and energy storage devices due to their environmental sustainability and resource renewability. However, preparing cellulose-based hydrogel electrolytes with super flexibility, high conductivity, and high specific capacitance for practical applications is still challenging. Herein, an adhesive, antibacterial, conductive zwitterionic cellulose nanofibersreinforced poly(sulfobetaine methacrylate-acrylic acid-acrylamide (ZCNF/PSAA) composite hydrogel was fabricated by a blue light-triggered free radical polymerization of 2-methacryloyloxy ethyl dimethyl-3sulfopropyl ammonium hydroxide (SBMA), acrylic acid (AA), acryl amide (AM), dopamine methacrylamide (DMA) and zwitterionic cellulose nanofibers (ZCNF). The prepared hydrogel exhibited excellent mechanical properties with tensile strength of 0.17 MPa, compressive strength of 0.87 MPa, and shear strength of 1.25 MPa, respectively. The zwitterionic groups significantly enhanced the hydrogel's conductivity (5.8 S/m). Moreover, the hydrogel with electrically sensitive perception of external strain (GF = 2.5), can withstand large bending and compression deformations and can be used as a motion sensor to monitor human movements such as arm and finger bending, pressing, and subtle fist clenching. The resulting hydrogel presented excellent antibacterial activity against Escherichia coli and Staphylococcus aureus. As the hydrogel was applied as electrolyte, the developed super-capacitor exhibited a desirable specific capacitance of 404.5 mF.cm-2, with a maximum energy density of 53.93 Wh.kg-1 and capacitance retention of 80.3 % after 2000 consecutive charge-discharge cycles. The ZCNF/ PSAA hydrogel has great potential for applications in flexible strain sensors and energy storage devices.
Keyword ：
Cellulose nanofibers Cellulose nanofibers Electrolytes Electrolytes Hydrogels Hydrogels Sensors Sensors Super-capacitors Super-capacitors Zwitterions Zwitterions
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| GB/T 7714 | Farooq, Ambar , Wanyan, Hongying , Li, Qin et al. An adhesive, antibacterial, conductive zwitterionic cellulose nanofibers-containing hydrogel for flexible strain sensors and super-capacitors [J]. | CARBOHYDRATE POLYMERS , 2025 , 358 . |
| MLA | Farooq, Ambar et al. "An adhesive, antibacterial, conductive zwitterionic cellulose nanofibers-containing hydrogel for flexible strain sensors and super-capacitors" . | CARBOHYDRATE POLYMERS 358 (2025) . |
| APA | Farooq, Ambar , Wanyan, Hongying , Li, Qin , Lu, Shengchang , Huang, Weiqi , Waqas, Muhammad et al. An adhesive, antibacterial, conductive zwitterionic cellulose nanofibers-containing hydrogel for flexible strain sensors and super-capacitors . | CARBOHYDRATE POLYMERS , 2025 , 358 . |
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The in-situ generation of hydrogen peroxide (H2O2) from oxygen and water with semiconductor photocatalysts under illumination is considered as a promising synthesis pathway. However, photocarrier recombination as well as slow transfer of charges involved in carbon nitride (C3N5, CN), are the enduring challenge for photocatalytic activity. Herein, we develop a pi-stacked CN-based composites (CNv-A) coupling natural polyphenolic anthocyanins (A) with defective carbon nitride (CNv) for efficient visible-light-driven H2O2 production. The strengthening pi-stacking (CNv-A) leads to extended electronic transmission networks via effective intermolecular pi-pi interactions, resulting in a high H2O2 generation rate of 147.2 mu mol.L-1.h-1, as well as 42 times that of the pristine CN. The combination of experimental results and theoretical calculations reveals that with the incorporation of anthocyanins, the intermolecular pi-pi stacking reconstructs the enlarged charge transfer networks over carbon nitride, thus facilitating electron transfer and active center dot O2- generation. Moreover, increasing the content of nitrogen vacancy of carbon nitride effectively strengthened the pi-pi interactions, accelerating the transfer and separation of charge carriers, thereby achieving drastic high-performance H2O2 production via an indirect single-electron oxygen reduction reaction (ORR) pathway. This work provides a new perspective for regulating charge transfer and separation by modulating the strength of intermolecular weak interactions.
Keyword ：
Anthocyanins Anthocyanins Carbon nitride Carbon nitride Charge transfer Charge transfer pi-pi stacking pi-pi stacking Vacancy engineering Vacancy engineering
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| GB/T 7714 | Wu, Shengye , Li, Yixi , Wei, Shuaichong et al. Coupling of anthocyanins at defective carbon nitride (C3N5) with π-π stacking for efficient photocatalytic H2O2 generation [J]. | CHEMICAL ENGINEERING JOURNAL , 2025 , 508 . |
| MLA | Wu, Shengye et al. "Coupling of anthocyanins at defective carbon nitride (C3N5) with π-π stacking for efficient photocatalytic H2O2 generation" . | CHEMICAL ENGINEERING JOURNAL 508 (2025) . |
| APA | Wu, Shengye , Li, Yixi , Wei, Shuaichong , Li, Jiashu , Zhang, Fengshan , Li, Jingde et al. Coupling of anthocyanins at defective carbon nitride (C3N5) with π-π stacking for efficient photocatalytic H2O2 generation . | CHEMICAL ENGINEERING JOURNAL , 2025 , 508 . |
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Hydrogen peroxide (H2O2) photosynthesis from oxygen and water has become an attracting route due to its green, low-carbon and sustainable features. Although carbon nitride (CN) is a remarkable semiconductor for photocatalytic H2O2 production, CN also suffers from slow transfer and poor separation efficiency of photogenerated charges due to the intrinsically molecular structures. Herein, we report a facile method to enhance H2O2 evolution with asymmetric CN via molten-salt assisted supramolecular assemblies of melamine and 2,4,6triaminopyrimidine (T). The optimum M-CNT exhibited a photocatalytic H2O2 production rate of 44.63 mu mol center dot L- 1h- 1, which is more than 4 times higher than that of pristine CN without any sacrificial agents. Experimental and DFT results demonstrate T molecule can tune the charge location of CN frameworks, promoting electron transfer and efficient separation. Furthermore, under the synergy of molten salt, the uneven distribution of intramolecular charges can be exacerbated to boost the photocatalytic performance through significant polarization effects. This work provided a paradigm of charge characteristics of carbon nitride via asymmetric molecular engineering for enhanced photocatalytic H2O2 generation.
Keyword ：
Asymmetric structure Asymmetric structure Carbon nitride Carbon nitride Hydrogen peroxide Hydrogen peroxide Photosynthesis Photosynthesis Polarization effect Polarization effect
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| GB/T 7714 | Li, Jiashu , Li, Yixi , Wei, Shuaichong et al. Asymmetric framework engineering of carbon nitride nanotubes for polarization promoted H2O2 photosynthesis [J]. | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY , 2025 , 366 . |
| MLA | Li, Jiashu et al. "Asymmetric framework engineering of carbon nitride nanotubes for polarization promoted H2O2 photosynthesis" . | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY 366 (2025) . |
| APA | Li, Jiashu , Li, Yixi , Wei, Shuaichong , Wu, Shengye , Peng, Zhangyan , Zhang, Fengshan et al. Asymmetric framework engineering of carbon nitride nanotubes for polarization promoted H2O2 photosynthesis . | APPLIED CATALYSIS B-ENVIRONMENT AND ENERGY , 2025 , 366 . |
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In this study, cellulose acetate (CA)-based polyamide (PA) nanofiltration membranes (CA-NF-2/0.4) with enhanced antifouling and separation performance were prepared through the interfacial polymerization of diethylenetriamine (DETA) and 1,3,5-benzenetricarbonyl chloride (TMC) for the effective removal of dyes and salt ions. Benefiting from the three reaction sites (primary and secondary amino groups) of DETA, a PA layer with a three-dimensional network structure formed on the CA substrate, imparting the CA-NF-2/0.4 membranes with a strong negative charge (-24.8 mV at pH 7) and a defect-free morphological feature. Consequently, the CA-NF-2/0.4 membranes exhibited high removal efficiencies for various dyes (99% for Rose Bengal and Congo Red, 95.5% for Methyl Orange, and 96.1% for Methylene Blue), as well as various monovalent and divalent salts, including MgCl2 (84.2%), Na2SO4 (92.7%), MgSO4 (91.8%), and NaCl (54.1%). Additionally, the CA-NF-2/0.4 membranes demonstrated excellent antifouling properties [the flux recovery ratio (flux recovery rate > 98.5%), long-term durability, and stability under high operational pressures and salt concentrations] due to their good hydrophilicity (water contact angle of 39.8 degrees) and the hydrogen bonding interaction between the active amine groups of DETA and the -OH groups of the CA support layer. This study presents an effective method for fabricating cellulose-based NF membranes with high separation and antifouling performance, offering insights into the high-value utilization of cellulose-based materials.
Keyword ：
antifouling antifouling cellulose acetate cellulose acetate diethylene triamine diethylene triamine nanofiltration membranes nanofiltration membranes three-dimensionalnetwork structure three-dimensionalnetwork structure
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| GB/T 7714 | Lin, Yaling , Mo, Minfu , Lin, Junkang et al. Cellulose Acetate-Based Polyamide Nanofiltration Membranes by Diethylenetriamine-Assisted Interfacial Polymerization for Effective Removal of Dyes and Salt Ions [J]. | ACS APPLIED POLYMER MATERIALS , 2025 , 7 (7) : 4153-4165 . |
| MLA | Lin, Yaling et al. "Cellulose Acetate-Based Polyamide Nanofiltration Membranes by Diethylenetriamine-Assisted Interfacial Polymerization for Effective Removal of Dyes and Salt Ions" . | ACS APPLIED POLYMER MATERIALS 7 . 7 (2025) : 4153-4165 . |
| APA | Lin, Yaling , Mo, Minfu , Lin, Junkang , Ma, Xiaojuan , Hong, Yubin , Chen, Lihui et al. Cellulose Acetate-Based Polyamide Nanofiltration Membranes by Diethylenetriamine-Assisted Interfacial Polymerization for Effective Removal of Dyes and Salt Ions . | ACS APPLIED POLYMER MATERIALS , 2025 , 7 (7) , 4153-4165 . |
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Batteries have become an integral part of today's life and are presented as the most appropriate approach for energy storage; however, the environmental impacts of their vast usage need to be considered. Therefore, it is essential to incorporate eco-friendly materials to design batteries. Cellulose, the most abundant natural polymer, comprises excellent physical, mechanical, and chemical properties. It presents a broad group of functional materials ranging from macro to nanoscale composites that exhibit their potential in energy-related fields. This review provides a comprehensive summary of structural features, the influence of cellulose-based materials on electrochemical performance, and potential applications of cellulose derivatives as separators, electrolytes, binders, and electrodes in advanced energy storage devices, including sodium-ion, zinc-ion, lithium-ion, and lithium-sulfur batteries and gives an insight of the effects of derivatization on application and electrochemical performance of batteries. This review aims to comprehensively understand the vast applications of cellulose derivatives as vital parts of batteries. At last, an outlook of the current issues and future challenges for applications of cellulose-based materials in batteries is presented.
Keyword ：
Batteries Batteries Binders Binders Cellulose Cellulose Electrode Electrode Electrolyte Electrolyte Separator Separator
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| GB/T 7714 | Farooq, Ambar , Wanyan, Hongying , Lu, Shengchang et al. A review on cellulose-based derivatives and composites for sustainable rechargeable batteries [J]. | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES , 2025 , 308 . |
| MLA | Farooq, Ambar et al. "A review on cellulose-based derivatives and composites for sustainable rechargeable batteries" . | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES 308 (2025) . |
| APA | Farooq, Ambar , Wanyan, Hongying , Lu, Shengchang , Mosisa, Mentgistu Tadesse , Zhou, Xiaxing , Xiao, He et al. A review on cellulose-based derivatives and composites for sustainable rechargeable batteries . | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES , 2025 , 308 . |
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The advancement of ecofriendly and high-performance energy transformation systems has driven the development of advanced membrane materials for alkaline water electrolysis (AWE), which conduct hydroxide ions and block the interpenetration of hydrogen and oxygen. The wettability and inadequate gas blocking remain challenges for the AWE membrane. In this study, a hydrophilic polyphenylene sulfide/cellulose/polyphenylene sulfide (PPS/C/PPS) composite membrane with high bubble point pressure (BPP), outstanding oxygen purity, and low area resistance (AR) was fabricated. The porous PPS/C/PPS membrane exhibits a high BPP of 12.4 bar and low AR of 0.014 Omegacm2. Notably, gas purity tests reveal that the oxygen purity is about 99.974%, which is much higher than that of commercial hydrophilic polyphenylene sulfide (C-HPPS) (98.5%). The AWE cell with the PPS/C/PPS composite membrane shows a current density (CD) of 319.2 mAcm-2 in 30 wt % KOH solution at 80 degrees C at a voltage of 2 V, surpassing that of C-HPPS (208.0 mAcm-2). Additionally, the AWE cell exhibits high stability of more than 450 h at KOH solution (30 wt %) without attenuation, emphasizing the membrane's competitive edge and its vast application potential.
Keyword ：
alkaline water electrolysis alkaline water electrolysis bubble point pressure bubble point pressure cellulose cellulose membrane membrane polyphenylene sulfide polyphenylene sulfide
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| GB/T 7714 | Huang, Jianhua , Zheng, Yulian , Wu, Hui et al. Hydrophilic Polyphenylene Sulfide/Cellulose/Polyphenylene Sulfide Composite Membrane with High Bubble Point Pressure and High Oxygen Purity for Alkaline Water Electrolysis [J]. | ACS APPLIED POLYMER MATERIALS , 2025 , 7 (7) : 4322-4328 . |
| MLA | Huang, Jianhua et al. "Hydrophilic Polyphenylene Sulfide/Cellulose/Polyphenylene Sulfide Composite Membrane with High Bubble Point Pressure and High Oxygen Purity for Alkaline Water Electrolysis" . | ACS APPLIED POLYMER MATERIALS 7 . 7 (2025) : 4322-4328 . |
| APA | Huang, Jianhua , Zheng, Yulian , Wu, Hui , Lin, Hui , Hong, Yubin , Chen, Lihui et al. Hydrophilic Polyphenylene Sulfide/Cellulose/Polyphenylene Sulfide Composite Membrane with High Bubble Point Pressure and High Oxygen Purity for Alkaline Water Electrolysis . | ACS APPLIED POLYMER MATERIALS , 2025 , 7 (7) , 4322-4328 . |
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Biochar materials, known for their low cost, abundant availability, green environmental protection and renewable nature, are extensively applied across the energy storage sector. However, their structure and inherent limitations of the raw materials greatly reduce their energy storage performance. In this research, we aimed to optimized the structure of Melaleuca leucadendron L. bark activated carbon (BAC) by adjusting the ball milling time and speed. We also explored the optimal composite mass ratio of BAC/polyaniline (PANI) and further enhanced the electrochemical performance of the pseudocapacitive material composite employing in-situ polymerization techniques with ferric chloride doping for PANI. The characterization of BAC/PANI composites was performed through scanning electron microscopy (SEM), nitrogen adsorption-desorption isotherms (BET), X-ray diffraction (XRD), and Fourier-transform infrared spectroscopy (FTIR). The BAC/PANI electrode materials' electrochemical capabilities and supercapacitor functionality were tested using cyclic voltammetry (CV), galvanostatic charge-discharge analysis (GCD), and electrochemical impedance spectroscopy (EIS). The study demonstrated that ball milling not only mended defects in amorphous carbon but also increased crystallinity and oxygen content. Additionally, the presence of PANI contributed nitrogen atoms. The functional groups with oxygen and nitrogen content improved the electrode materials' wettability, which contributed to the pseudo-capacitive effect and subsequently increased electrochemical performance. The BAC/PANI-FeCl3-10 material exhibits a defined capacitance of 414.0 F g-1 at a current density of 0.5 A g-1, and maintained a capacity retention rate of 74.7 % after 5000 cycles, with an energy density output of 5.2 Wh kg-1 at a high-power density of 1872.0 W kg-1. © 2025, The Authors. All rights reserved.
Keyword ：
Adsorption isotherms Adsorption isotherms Carbon carbon composites Carbon carbon composites Crystallinity Crystallinity Cyclic voltammetry Cyclic voltammetry Fourier transform infrared spectroscopy Fourier transform infrared spectroscopy Gas adsorption Gas adsorption Semiconductor doping Semiconductor doping
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| GB/T 7714 | Yu, Ting , Zhang, Peiyuan , Chen, Lihui et al. Preparation of High-Performance Supercapacitors Using Bark Activated Carbon/Polyaniline Composite Electrode [J]. | SSRN , 2025 . |
| MLA | Yu, Ting et al. "Preparation of High-Performance Supercapacitors Using Bark Activated Carbon/Polyaniline Composite Electrode" . | SSRN (2025) . |
| APA | Yu, Ting , Zhang, Peiyuan , Chen, Lihui , Huang, Liulian , Wu, Hui , Zhou, Xiaxing . Preparation of High-Performance Supercapacitors Using Bark Activated Carbon/Polyaniline Composite Electrode . | SSRN , 2025 . |
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As a natural polymer, cellulose has emerged as a promising candidate for constructing versatile materials and products due to its intrinsic biocompatibility, environmental degradability, and structural stability. As a state-ofthe-art output, cellulose ionogel has demonstrated advanced applications in various scenarios in the Internet-of-Things era, while the weak mechanical strength is significantly challenging. To address this limitation, we developed a simple self-crosslinked stagey of cellulose molecules by triggering the chemical reactions of the hydroxyl and dialdehyde groups. Such chemical bonds between cellulose molecules create the tough selfcrosslinked cellulose-ionogel (SCCell-ionogel), which demonstrates super high strength of 4.23 MPa with 540 % improvement, toughness of 1.36 MJ/m3 with a 900 % increase. In addition, the resultant SCCell-ionogel also features high transmittance (93 %) and desirable biodegradation. The self-crosslinked strategy paves the way for constructing high-performance, advanced ionogel of natural polymer for next-generation smart materials.
Keyword ：
Dialdehyde cellulose Dialdehyde cellulose Ionogel Ionogel Self-crosslinked Self-crosslinked Toughness Toughness
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| GB/T 7714 | Li, Qingyuan , Yang, Jiawei , Zheng, Xiaobin et al. Self-crosslinked cellulose for tough ionogel [J]. | INDUSTRIAL CROPS AND PRODUCTS , 2025 , 229 . |
| MLA | Li, Qingyuan et al. "Self-crosslinked cellulose for tough ionogel" . | INDUSTRIAL CROPS AND PRODUCTS 229 (2025) . |
| APA | Li, Qingyuan , Yang, Jiawei , Zheng, Xiaobin , Wu, Hui , Huang, Liulian , Zhao, He et al. Self-crosslinked cellulose for tough ionogel . | INDUSTRIAL CROPS AND PRODUCTS , 2025 , 229 . |
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Biochar materials, known for their low cost, abundant availability, green environmental protection and renewable nature, are extensively applied across the energy storage sector. However, their structure and inherent limitations of the raw materials greatly reduce their energy storage performance. In this research, we aimed to optimized the structure of Melaleuca leucadendron L. bark activated carbon (BAC) by adjusting the ball milling time and speed. We also explored the optimal composite mass ratio of BAC/polyaniline (PANI) and further enhanced the electrochemical performance of the pseudocapacitive material composite employing in-situ polymerization techniques with ferric chloride doping for PANI. The characterization of BAC/PANI composites was performed through scanning electron microscopy (SEM), nitrogen adsorption-desorption isotherms (BET), X-ray diffraction (XRD), and Fourier-transform infrared spectroscopy (FTIR). The BAC/PANI electrode materials' electrochemical capabilities and supercapacitor functionality were tested using cyclic voltammetry (CV), galvanostatic charge-discharge analysis (GCD), and electrochemical impedance spectroscopy (EIS). The study demonstrated that ball milling not only mended defects in amorphous carbon but also increased crystallinity and oxygen content. Additionally, the presence of PANI contributed nitrogen atoms. The functional groups with oxygen and nitrogen content improved the electrode materials' wettability, which contributed to the pseudo-capacitive effect and subsequently increased electrochemical performance. The BAC/PANI-FeCl3-10 material exhibits a defined capacitance of 414.0 F g- 1 at a current density of 0.5 A g- 1, and maintained a capacity retention rate of 74.7 % after 5000 cycles, with an energy density output of 5.2 Wh kg- 1 at a high-power density of 1872.0 W kg- 1. This research provides a theoretical and empirical foundation for the utilization of bark activated carbon as an electrode material in supercapacitors, paving the way for more efficient and sustainable energy storage solutions.
Keyword ：
Biochar material Biochar material Melaleuca leucadendron L. bark Melaleuca leucadendron L. bark Polyaniline Polyaniline Supercapacitor Supercapacitor
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| GB/T 7714 | Yu, Ting , Zhang, Peiyuan , Chen, Lihui et al. Preparation of high-performance supercapacitors using bark activated carbon/polyaniline composite electrode [J]. | BIOMASS & BIOENERGY , 2025 , 197 . |
| MLA | Yu, Ting et al. "Preparation of high-performance supercapacitors using bark activated carbon/polyaniline composite electrode" . | BIOMASS & BIOENERGY 197 (2025) . |
| APA | Yu, Ting , Zhang, Peiyuan , Chen, Lihui , Huang, Liulian , Wu, Hui , Zhou, Xiaxing . Preparation of high-performance supercapacitors using bark activated carbon/polyaniline composite electrode . | BIOMASS & BIOENERGY , 2025 , 197 . |
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Flexible hybrid nanogenerators (HNGs) have received significant attention for their potential in harvesting mechanical energy to power portable and miniaturized portable devices. This work presents a method to fabricate flexible, durable and biodegradable electrospun polydopamine@barium titanate/cellulose acetate (PDA@BTO/CA) nanofiber films. This design integrates polydopamine (PDA) and piezoelectric barium titanate (BTO) nanoparticles within a flexible cellulose acetate (CA) matrix to enable self-powered wearable biomonitoring. The inclusion of PDA enhances the physical adhesion between BTO and CA, resulting in a significant 40% increase in voltage output. Notably, the PDA-modified composite PDA@BTO/CA demonstrates remarkable durability over 15,000 cycles and effectively detects a range of human motions (such as fist clenching, wrist bending, elbow movement, walking, running and jumping), transducing them into stable, precise electrical signals. Intriguingly, the hybrid nanogenerator device exhibits robust performance in extreme conditions, including underwater and high or low temperatures, while maintaining its good biodegradability. This work paves the way for advanced self-powered wearable biosensor devices capable of precise and reliable human motion monitoring.
Keyword ：
Cellulose Cellulose Composite Composite Hybrid nanogenerator Hybrid nanogenerator Polydopamine Polydopamine Wearable sensors Wearable sensors
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| GB/T 7714 | Lu, Shengchang , Li, Shuai , Li, Qin et al. Flexible cellulose-based hybrid nanogenerators for self-powered wearable bio-monitoring applications [J]. | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2025 , 685 : 1087-1098 . |
| MLA | Lu, Shengchang et al. "Flexible cellulose-based hybrid nanogenerators for self-powered wearable bio-monitoring applications" . | JOURNAL OF COLLOID AND INTERFACE SCIENCE 685 (2025) : 1087-1098 . |
| APA | Lu, Shengchang , Li, Shuai , Li, Qin , Yang, Lin , Zhang, Hui , Li, Jianguo et al. Flexible cellulose-based hybrid nanogenerators for self-powered wearable bio-monitoring applications . | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2025 , 685 , 1087-1098 . |
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