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学者姓名：吴慧
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Abstract ：
Adhesive patches are optimum candidates for distinct biomedical applications, including tissue adhesion and leakage sealing in outpatient or surgical procedures. Unfortunately, most adhesive patches are significantly less effective at providing strong adhesion to the surface of wet tissue, which increases the risk and reduces the fault tolerance in surgery. Meanwhile, customization is difficult to achieve in terms of mechanical adaptability. To tackle this problem, we developed a chitosan-containing bioadhesive patch (ANC) comprising dual-crosslinked carboxymethyl chitosan methacrylate (CMCS-MA), acrylic acid, and acrylic acid N-hydroxysuccinimide ester. This ingenious and convenient design strategy facilitates the integrated polymerization of the patch, while circumventing the necessity for additional crosslinkers. ANC patches in dry state and the rich carboxyl groups contained therein enable rapid removal of moisture from tissue surfaces. Subsequently, robust adhesion based on hydrogen bonding and N-hydroxysuccinimide (NHS)-amine interaction is formed. The dual-crosslinked ANC patch achieves good adjustable mechanical performance and swelling behavior by controlling the addition of CMCS-MA. Furthermore, compared with commercially available fibrin glue, ANC patches own robust adhesion and superior sealing performance for stomach fluid leakage. This intricately designed ANC patch sheds new light on biomedical patch design and broadens the scope of chitosan-containing materials in tissue adhesive and sealant applications.
Keyword ：
adhesive adhesive chitosan chitosan dual-crosslinked dual-crosslinked patch patch
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| GB/T 7714 | Yang, Jiayu , Li, Qiaoling , Zhang, Jianpeng et al. A Chitosan-Containing Dual-Crosslinked Resilient Patch for Tissue Adhesive and Sealant [J]. | CHEMISTRY & BIODIVERSITY , 2025 , 22 (9) . |
| MLA | Yang, Jiayu et al. "A Chitosan-Containing Dual-Crosslinked Resilient Patch for Tissue Adhesive and Sealant" . | CHEMISTRY & BIODIVERSITY 22 . 9 (2025) . |
| APA | Yang, Jiayu , Li, Qiaoling , Zhang, Jianpeng , Wu, Siyang , Zhang, Min , Chen, Lihui et al. A Chitosan-Containing Dual-Crosslinked Resilient Patch for Tissue Adhesive and Sealant . | CHEMISTRY & BIODIVERSITY , 2025 , 22 (9) . |
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Cellulose-based hydrogels are promising materials for constructing flexible supercapacitors and energy storage devices due to their environmental sustainability and resource renewability. However, preparing cellulose-based hydrogel electrolytes with super flexibility, high conductivity, and high specific capacitance for practical applications is still challenging. Herein, an adhesive, antibacterial, conductive zwitterionic cellulose nanofibersreinforced poly(sulfobetaine methacrylate-acrylic acid-acrylamide (ZCNF/PSAA) composite hydrogel was fabricated by a blue light-triggered free radical polymerization of 2-methacryloyloxy ethyl dimethyl-3sulfopropyl ammonium hydroxide (SBMA), acrylic acid (AA), acryl amide (AM), dopamine methacrylamide (DMA) and zwitterionic cellulose nanofibers (ZCNF). The prepared hydrogel exhibited excellent mechanical properties with tensile strength of 0.17 MPa, compressive strength of 0.87 MPa, and shear strength of 1.25 MPa, respectively. The zwitterionic groups significantly enhanced the hydrogel's conductivity (5.8 S/m). Moreover, the hydrogel with electrically sensitive perception of external strain (GF = 2.5), can withstand large bending and compression deformations and can be used as a motion sensor to monitor human movements such as arm and finger bending, pressing, and subtle fist clenching. The resulting hydrogel presented excellent antibacterial activity against Escherichia coli and Staphylococcus aureus. As the hydrogel was applied as electrolyte, the developed super-capacitor exhibited a desirable specific capacitance of 404.5 mF.cm-2, with a maximum energy density of 53.93 Wh.kg-1 and capacitance retention of 80.3 % after 2000 consecutive charge-discharge cycles. The ZCNF/ PSAA hydrogel has great potential for applications in flexible strain sensors and energy storage devices.
Keyword ：
Cellulose nanofibers Cellulose nanofibers Electrolytes Electrolytes Hydrogels Hydrogels Sensors Sensors Super-capacitors Super-capacitors Zwitterions Zwitterions
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| GB/T 7714 | Farooq, Ambar , Wanyan, Hongying , Li, Qin et al. An adhesive, antibacterial, conductive zwitterionic cellulose nanofibers-containing hydrogel for flexible strain sensors and super-capacitors [J]. | CARBOHYDRATE POLYMERS , 2025 , 358 . |
| MLA | Farooq, Ambar et al. "An adhesive, antibacterial, conductive zwitterionic cellulose nanofibers-containing hydrogel for flexible strain sensors and super-capacitors" . | CARBOHYDRATE POLYMERS 358 (2025) . |
| APA | Farooq, Ambar , Wanyan, Hongying , Li, Qin , Lu, Shengchang , Huang, Weiqi , Waqas, Muhammad et al. An adhesive, antibacterial, conductive zwitterionic cellulose nanofibers-containing hydrogel for flexible strain sensors and super-capacitors . | CARBOHYDRATE POLYMERS , 2025 , 358 . |
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Batteries have become an integral part of today's life and are presented as the most appropriate approach for energy storage; however, the environmental impacts of their vast usage need to be considered. Therefore, it is essential to incorporate eco-friendly materials to design batteries. Cellulose, the most abundant natural polymer, comprises excellent physical, mechanical, and chemical properties. It presents a broad group of functional materials ranging from macro to nanoscale composites that exhibit their potential in energy-related fields. This review provides a comprehensive summary of structural features, the influence of cellulose-based materials on electrochemical performance, and potential applications of cellulose derivatives as separators, electrolytes, binders, and electrodes in advanced energy storage devices, including sodium-ion, zinc-ion, lithium-ion, and lithium-sulfur batteries and gives an insight of the effects of derivatization on application and electrochemical performance of batteries. This review aims to comprehensively understand the vast applications of cellulose derivatives as vital parts of batteries. At last, an outlook of the current issues and future challenges for applications of cellulose-based materials in batteries is presented.
Keyword ：
Batteries Batteries Binders Binders Cellulose Cellulose Electrode Electrode Electrolyte Electrolyte Separator Separator
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| GB/T 7714 | Farooq, Ambar , Wanyan, Hongying , Lu, Shengchang et al. A review on cellulose-based derivatives and composites for sustainable rechargeable batteries [J]. | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES , 2025 , 308 . |
| MLA | Farooq, Ambar et al. "A review on cellulose-based derivatives and composites for sustainable rechargeable batteries" . | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES 308 (2025) . |
| APA | Farooq, Ambar , Wanyan, Hongying , Lu, Shengchang , Mosisa, Mentgistu Tadesse , Zhou, Xiaxing , Xiao, He et al. A review on cellulose-based derivatives and composites for sustainable rechargeable batteries . | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES , 2025 , 308 . |
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High locoregional recurrence rates and potential wound infections remain a significant challenge for postoperative breast cancer patients. Herein, we developed a dual-network hyaluronic acid (HA) nanocomposite hydrogel composed of herring sperm DNA (hsDNA) bridged methacrylated HA (HAMA) and FeMg-LDH-ppsa nanohybrid chelated catechol-modified HA (HADA) for the prevention of breast cancer recurrent, antiinfection, and promoting wound healing. Dynamic reversible hsDNA cross-linking combined with metalcatechol chelating renders the hydrogel injectability, rapid self-healing ability, and enhanced mechanical properties. FeMg-LDH-ppsa nanohybrids obtained by in situ polymerization of aniline derivatives in the FeMgLDH interlayer exhibited excellent photothermal effect. Upon near-infrared (NIR) irradiation, the photothermal effect mediated by FeMg-LDH-ppsa can unwind the hsDNA duplex, enabling the controlled release of preloaded DOX for synergistic photothermal-chemotherapy antitumor. Meanwhile, the catechol-metal (Fe3+/ Mg2+) moieties in the hydrogel enhanced tissue adhesion and exhibited intrinsic antimicrobial and bioactive properties, which in combination with the NIR-assisted photothermal effect, significantly accelerated infected wound healing through sterilizing microorganisms, alleviating inflammation, re-epithelialization, and angiogenesis. Overall, this multifunctional hydrogel represented a promising candidate in postoperative wound management for simultaneous tumor elimination, antiinfection, and wound repair.
Keyword ：
Dynamic dual-crosslinking network Dynamic dual-crosslinking network NIR-triggered drug release NIR-triggered drug release Photothermal nanohybrid Photothermal nanohybrid Postoperative tumor therapy Postoperative tumor therapy Space-confined polymerization Space-confined polymerization
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| GB/T 7714 | Zhang, Yu , Li, Lixia , Jiang, Xiaohe et al. Injectable dual-network hyaluronic acid nanocomposite hydrogel for prevention of postoperative breast cancer recurrence and wound healing [J]. | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES , 2025 , 291 . |
| MLA | Zhang, Yu et al. "Injectable dual-network hyaluronic acid nanocomposite hydrogel for prevention of postoperative breast cancer recurrence and wound healing" . | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES 291 (2025) . |
| APA | Zhang, Yu , Li, Lixia , Jiang, Xiaohe , Liu, Haimeng , Guo, Xiaolu , Wu, Hui et al. Injectable dual-network hyaluronic acid nanocomposite hydrogel for prevention of postoperative breast cancer recurrence and wound healing . | INTERNATIONAL JOURNAL OF BIOLOGICAL MACROMOLECULES , 2025 , 291 . |
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The advancement of ecofriendly and high-performance energy transformation systems has driven the development of advanced membrane materials for alkaline water electrolysis (AWE), which conduct hydroxide ions and block the interpenetration of hydrogen and oxygen. The wettability and inadequate gas blocking remain challenges for the AWE membrane. In this study, a hydrophilic polyphenylene sulfide/cellulose/polyphenylene sulfide (PPS/C/PPS) composite membrane with high bubble point pressure (BPP), outstanding oxygen purity, and low area resistance (AR) was fabricated. The porous PPS/C/PPS membrane exhibits a high BPP of 12.4 bar and low AR of 0.014 Omegacm2. Notably, gas purity tests reveal that the oxygen purity is about 99.974%, which is much higher than that of commercial hydrophilic polyphenylene sulfide (C-HPPS) (98.5%). The AWE cell with the PPS/C/PPS composite membrane shows a current density (CD) of 319.2 mAcm-2 in 30 wt % KOH solution at 80 degrees C at a voltage of 2 V, surpassing that of C-HPPS (208.0 mAcm-2). Additionally, the AWE cell exhibits high stability of more than 450 h at KOH solution (30 wt %) without attenuation, emphasizing the membrane's competitive edge and its vast application potential.
Keyword ：
alkaline water electrolysis alkaline water electrolysis bubble point pressure bubble point pressure cellulose cellulose membrane membrane polyphenylene sulfide polyphenylene sulfide
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| GB/T 7714 | Huang, Jianhua , Zheng, Yulian , Wu, Hui et al. Hydrophilic Polyphenylene Sulfide/Cellulose/Polyphenylene Sulfide Composite Membrane with High Bubble Point Pressure and High Oxygen Purity for Alkaline Water Electrolysis [J]. | ACS APPLIED POLYMER MATERIALS , 2025 , 7 (7) : 4322-4328 . |
| MLA | Huang, Jianhua et al. "Hydrophilic Polyphenylene Sulfide/Cellulose/Polyphenylene Sulfide Composite Membrane with High Bubble Point Pressure and High Oxygen Purity for Alkaline Water Electrolysis" . | ACS APPLIED POLYMER MATERIALS 7 . 7 (2025) : 4322-4328 . |
| APA | Huang, Jianhua , Zheng, Yulian , Wu, Hui , Lin, Hui , Hong, Yubin , Chen, Lihui et al. Hydrophilic Polyphenylene Sulfide/Cellulose/Polyphenylene Sulfide Composite Membrane with High Bubble Point Pressure and High Oxygen Purity for Alkaline Water Electrolysis . | ACS APPLIED POLYMER MATERIALS , 2025 , 7 (7) , 4322-4328 . |
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Biochar materials, known for their low cost, abundant availability, green environmental protection and renewable nature, are extensively applied across the energy storage sector. However, their structure and inherent limitations of the raw materials greatly reduce their energy storage performance. In this research, we aimed to optimized the structure of Melaleuca leucadendron L. bark activated carbon (BAC) by adjusting the ball milling time and speed. We also explored the optimal composite mass ratio of BAC/polyaniline (PANI) and further enhanced the electrochemical performance of the pseudocapacitive material composite employing in-situ polymerization techniques with ferric chloride doping for PANI. The characterization of BAC/PANI composites was performed through scanning electron microscopy (SEM), nitrogen adsorption-desorption isotherms (BET), X-ray diffraction (XRD), and Fourier-transform infrared spectroscopy (FTIR). The BAC/PANI electrode materials' electrochemical capabilities and supercapacitor functionality were tested using cyclic voltammetry (CV), galvanostatic charge-discharge analysis (GCD), and electrochemical impedance spectroscopy (EIS). The study demonstrated that ball milling not only mended defects in amorphous carbon but also increased crystallinity and oxygen content. Additionally, the presence of PANI contributed nitrogen atoms. The functional groups with oxygen and nitrogen content improved the electrode materials' wettability, which contributed to the pseudo-capacitive effect and subsequently increased electrochemical performance. The BAC/PANI-FeCl3-10 material exhibits a defined capacitance of 414.0 F g-1 at a current density of 0.5 A g-1, and maintained a capacity retention rate of 74.7 % after 5000 cycles, with an energy density output of 5.2 Wh kg-1 at a high-power density of 1872.0 W kg-1. © 2025, The Authors. All rights reserved.
Keyword ：
Adsorption isotherms Adsorption isotherms Carbon carbon composites Carbon carbon composites Crystallinity Crystallinity Cyclic voltammetry Cyclic voltammetry Fourier transform infrared spectroscopy Fourier transform infrared spectroscopy Gas adsorption Gas adsorption Semiconductor doping Semiconductor doping
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| GB/T 7714 | Yu, Ting , Zhang, Peiyuan , Chen, Lihui et al. Preparation of High-Performance Supercapacitors Using Bark Activated Carbon/Polyaniline Composite Electrode [J]. | SSRN , 2025 . |
| MLA | Yu, Ting et al. "Preparation of High-Performance Supercapacitors Using Bark Activated Carbon/Polyaniline Composite Electrode" . | SSRN (2025) . |
| APA | Yu, Ting , Zhang, Peiyuan , Chen, Lihui , Huang, Liulian , Wu, Hui , Zhou, Xiaxing . Preparation of High-Performance Supercapacitors Using Bark Activated Carbon/Polyaniline Composite Electrode . | SSRN , 2025 . |
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As a natural polymer, cellulose has emerged as a promising candidate for constructing versatile materials and products due to its intrinsic biocompatibility, environmental degradability, and structural stability. As a state-ofthe-art output, cellulose ionogel has demonstrated advanced applications in various scenarios in the Internet-of-Things era, while the weak mechanical strength is significantly challenging. To address this limitation, we developed a simple self-crosslinked stagey of cellulose molecules by triggering the chemical reactions of the hydroxyl and dialdehyde groups. Such chemical bonds between cellulose molecules create the tough selfcrosslinked cellulose-ionogel (SCCell-ionogel), which demonstrates super high strength of 4.23 MPa with 540 % improvement, toughness of 1.36 MJ/m3 with a 900 % increase. In addition, the resultant SCCell-ionogel also features high transmittance (93 %) and desirable biodegradation. The self-crosslinked strategy paves the way for constructing high-performance, advanced ionogel of natural polymer for next-generation smart materials.
Keyword ：
Dialdehyde cellulose Dialdehyde cellulose Ionogel Ionogel Self-crosslinked Self-crosslinked Toughness Toughness
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| GB/T 7714 | Li, Qingyuan , Yang, Jiawei , Zheng, Xiaobin et al. Self-crosslinked cellulose for tough ionogel [J]. | INDUSTRIAL CROPS AND PRODUCTS , 2025 , 229 . |
| MLA | Li, Qingyuan et al. "Self-crosslinked cellulose for tough ionogel" . | INDUSTRIAL CROPS AND PRODUCTS 229 (2025) . |
| APA | Li, Qingyuan , Yang, Jiawei , Zheng, Xiaobin , Wu, Hui , Huang, Liulian , Zhao, He et al. Self-crosslinked cellulose for tough ionogel . | INDUSTRIAL CROPS AND PRODUCTS , 2025 , 229 . |
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Biochar materials, known for their low cost, abundant availability, green environmental protection and renewable nature, are extensively applied across the energy storage sector. However, their structure and inherent limitations of the raw materials greatly reduce their energy storage performance. In this research, we aimed to optimized the structure of Melaleuca leucadendron L. bark activated carbon (BAC) by adjusting the ball milling time and speed. We also explored the optimal composite mass ratio of BAC/polyaniline (PANI) and further enhanced the electrochemical performance of the pseudocapacitive material composite employing in-situ polymerization techniques with ferric chloride doping for PANI. The characterization of BAC/PANI composites was performed through scanning electron microscopy (SEM), nitrogen adsorption-desorption isotherms (BET), X-ray diffraction (XRD), and Fourier-transform infrared spectroscopy (FTIR). The BAC/PANI electrode materials' electrochemical capabilities and supercapacitor functionality were tested using cyclic voltammetry (CV), galvanostatic charge-discharge analysis (GCD), and electrochemical impedance spectroscopy (EIS). The study demonstrated that ball milling not only mended defects in amorphous carbon but also increased crystallinity and oxygen content. Additionally, the presence of PANI contributed nitrogen atoms. The functional groups with oxygen and nitrogen content improved the electrode materials' wettability, which contributed to the pseudo-capacitive effect and subsequently increased electrochemical performance. The BAC/PANI-FeCl3-10 material exhibits a defined capacitance of 414.0 F g- 1 at a current density of 0.5 A g- 1, and maintained a capacity retention rate of 74.7 % after 5000 cycles, with an energy density output of 5.2 Wh kg- 1 at a high-power density of 1872.0 W kg- 1. This research provides a theoretical and empirical foundation for the utilization of bark activated carbon as an electrode material in supercapacitors, paving the way for more efficient and sustainable energy storage solutions.
Keyword ：
Biochar material Biochar material Melaleuca leucadendron L. bark Melaleuca leucadendron L. bark Polyaniline Polyaniline Supercapacitor Supercapacitor
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| GB/T 7714 | Yu, Ting , Zhang, Peiyuan , Chen, Lihui et al. Preparation of high-performance supercapacitors using bark activated carbon/polyaniline composite electrode [J]. | BIOMASS & BIOENERGY , 2025 , 197 . |
| MLA | Yu, Ting et al. "Preparation of high-performance supercapacitors using bark activated carbon/polyaniline composite electrode" . | BIOMASS & BIOENERGY 197 (2025) . |
| APA | Yu, Ting , Zhang, Peiyuan , Chen, Lihui , Huang, Liulian , Wu, Hui , Zhou, Xiaxing . Preparation of high-performance supercapacitors using bark activated carbon/polyaniline composite electrode . | BIOMASS & BIOENERGY , 2025 , 197 . |
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Flexible hybrid nanogenerators (HNGs) have received significant attention for their potential in harvesting mechanical energy to power portable and miniaturized portable devices. This work presents a method to fabricate flexible, durable and biodegradable electrospun polydopamine@barium titanate/cellulose acetate (PDA@BTO/CA) nanofiber films. This design integrates polydopamine (PDA) and piezoelectric barium titanate (BTO) nanoparticles within a flexible cellulose acetate (CA) matrix to enable self-powered wearable biomonitoring. The inclusion of PDA enhances the physical adhesion between BTO and CA, resulting in a significant 40% increase in voltage output. Notably, the PDA-modified composite PDA@BTO/CA demonstrates remarkable durability over 15,000 cycles and effectively detects a range of human motions (such as fist clenching, wrist bending, elbow movement, walking, running and jumping), transducing them into stable, precise electrical signals. Intriguingly, the hybrid nanogenerator device exhibits robust performance in extreme conditions, including underwater and high or low temperatures, while maintaining its good biodegradability. This work paves the way for advanced self-powered wearable biosensor devices capable of precise and reliable human motion monitoring.
Keyword ：
Cellulose Cellulose Composite Composite Hybrid nanogenerator Hybrid nanogenerator Polydopamine Polydopamine Wearable sensors Wearable sensors
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| GB/T 7714 | Lu, Shengchang , Li, Shuai , Li, Qin et al. Flexible cellulose-based hybrid nanogenerators for self-powered wearable bio-monitoring applications [J]. | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2025 , 685 : 1087-1098 . |
| MLA | Lu, Shengchang et al. "Flexible cellulose-based hybrid nanogenerators for self-powered wearable bio-monitoring applications" . | JOURNAL OF COLLOID AND INTERFACE SCIENCE 685 (2025) : 1087-1098 . |
| APA | Lu, Shengchang , Li, Shuai , Li, Qin , Yang, Lin , Zhang, Hui , Li, Jianguo et al. Flexible cellulose-based hybrid nanogenerators for self-powered wearable bio-monitoring applications . | JOURNAL OF COLLOID AND INTERFACE SCIENCE , 2025 , 685 , 1087-1098 . |
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With the flourishing of mussel-inspired chemistry, the fast-growing development for environmentally friendly materials, and the need for inexpensive and biocompatible analogues to PDA in gel design, TA has led to its gradual emergence as a research focus due to its remarkable biocompatible, renewable, sustainable and particular physicochemical properties. As a natural building block, TA can be used as a substrate or crosslinker, ensuring versatile functional polymeric networks for various applications. In this review, the design of TA-based gels is summarized in detail (i.e., different interactions such as: metal coordination, electrostatic, hydrophobic, host-guest, cation-pi and pi-pi stacking interactions, hydrogen bonding and various reactions including: phenol-amine Michael and Schiff base, phenol-thiol Michael addition, phenol-epoxy ring opening reaction, etc.). Subsequently, TA-based gels with a variety of functionalities, including mechanical, adhesion, conductive, self-healing, UV-shielding, anti-swelling, anti-freezing, shape memory, antioxidant, antibacterial, anti-inflammatory and responsive properties are introduced in detail. Then, a summary of recent developments in the use of TA-based gels is provided, including bioelectronics, biomedicine, energy, packaging, water treatment and other fields. Finally, the difficulties that TA-based gels are currently facing are outlined, and an original yet realistic viewpoint is provided in an effort to spur future development.
Keyword ：
Applications Applications Design Design Gels Gels Properties Properties Tannic acid Tannic acid
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| GB/T 7714 | Tang, Zuwu , Chowdhury, Ilnaz Fargul , Yang, Jinbei et al. Recent advances in tannic acid-based gels: Design, properties, and applications [J]. | ADVANCES IN COLLOID AND INTERFACE SCIENCE , 2025 , 339 . |
| MLA | Tang, Zuwu et al. "Recent advances in tannic acid-based gels: Design, properties, and applications" . | ADVANCES IN COLLOID AND INTERFACE SCIENCE 339 (2025) . |
| APA | Tang, Zuwu , Chowdhury, Ilnaz Fargul , Yang, Jinbei , Li, Shi , Mondal, Ajoy Kanti , Wu, Hui . Recent advances in tannic acid-based gels: Design, properties, and applications . | ADVANCES IN COLLOID AND INTERFACE SCIENCE , 2025 , 339 . |
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