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学者姓名：赵雨萌
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Abstract ：
Significant progress has been made in recent years in the development of high-performance lithium batteries, which are critical to meeting the growing demands for next-generation energy storage systems, wide range of electronic devices and technological applications. Solid-state lithium metal batteries (SSLMBs) are considered as one of the most promising alternatives to state-of-the-art lithium-ion batteries (LIBs) due to their potential for higher energy density and the ability to address safety concerns associated with traditional LIBs that use flammable liquid electrolytes. Despite their promise, SSLMBs still face significant challenges that hinder their practical application, particularly in terms of Li+ conductivity, Li+ transference number, thickness, machinability, mechanochemical stability, and interfacial compatibility. This review comprehensively examined the specific properties of practical solid-state electrolytes (SSEs) based on current applications and summarized the opportunities and challenges in designing high-performance SSEs with high Li+ conductivity, high Li+ transference number, and ultra-thin structures (referred to as HCTSEs). Furthermore, the advantages and limitations of various design strategies were discussed and evaluated. The performance improvements of SSLMBs enabled by HCTSEs were summarized, and new perspectives on the design of HCTSEs were proposed to facilitate the largescale application of SSLMBs in the future.
Keyword ：
High Li+ conductivity High Li+ conductivity High Li+ transfer number High Li+ transfer number High-performance lithium batteries High-performance lithium batteries Solid-state electrolyte Solid-state electrolyte Ultrathin Ultrathin
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| GB/T 7714 | Tang, Wenjing , Zhao, Yumeng , Fu, Yu et al. Ultra-thin, high-performance composite solid electrolytes for lithium metal batteries: Progress and prospects [J]. | ENERGY STORAGE MATERIALS , 2025 , 79 . |
| MLA | Tang, Wenjing et al. "Ultra-thin, high-performance composite solid electrolytes for lithium metal batteries: Progress and prospects" . | ENERGY STORAGE MATERIALS 79 (2025) . |
| APA | Tang, Wenjing , Zhao, Yumeng , Fu, Yu , Wang, Aoxuan , Wu, Wei , Li, Wensong et al. Ultra-thin, high-performance composite solid electrolytes for lithium metal batteries: Progress and prospects . | ENERGY STORAGE MATERIALS , 2025 , 79 . |
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| GB/T 7714 | Zhao, Yumeng , Li, Changdong , Xu, Dehua et al. 900 Wh L–1 lithium-ion batteries enabled by self-assembled copolymer induced built-in electric field on graphite anode [J]. | Science Bulletin , 2025 . |
| MLA | Zhao, Yumeng et al. "900 Wh L–1 lithium-ion batteries enabled by self-assembled copolymer induced built-in electric field on graphite anode" . | Science Bulletin (2025) . |
| APA | Zhao, Yumeng , Li, Changdong , Xu, Dehua , Li, Rui , Han, Bin , Chen, Xinlian et al. 900 Wh L–1 lithium-ion batteries enabled by self-assembled copolymer induced built-in electric field on graphite anode . | Science Bulletin , 2025 . |
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